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基于地面的移动测量,以追踪八国12个城市天然气产生的城市甲烷排放。

Ground-Based Mobile Measurements to Track Urban Methane Emissions from Natural Gas in 12 Cities across Eight Countries.

作者信息

Vogel F, Ars S, Wunch D, Lavoie J, Gillespie L, Maazallahi H, Röckmann T, Nęcki J, Bartyzel J, Jagoda P, Lowry D, France J, Fernandez J, Bakkaloglu S, Fisher R, Lanoiselle M, Chen H, Oudshoorn M, Yver-Kwok C, Defratyka S, Morgui J A, Estruch C, Curcoll R, Grossi C, Chen J, Dietrich F, Forstmaier A, Denier van der Gon H A C, Dellaert S N C, Salo J, Corbu M, Iancu S S, Tudor A S, Scarlat A I, Calcan A

机构信息

Climate Research Division, Environment and Climate Change Canada, Toronto M3H 5T4, Canada.

Department of Physics, University of Toronto, Toronto M5S 1A7, Canada.

出版信息

Environ Sci Technol. 2024 Feb 6;58(5):2271-2281. doi: 10.1021/acs.est.3c03160. Epub 2024 Jan 25.

Abstract

To mitigate methane emission from urban natural gas distribution systems, it is crucial to understand local leak rates and occurrence rates. To explore urban methane emissions in cities outside the U.S., where significant emissions were found previously, mobile measurements were performed in 12 cities across eight countries. The surveyed cities range from medium size, like Groningen, NL, to large size, like Toronto, CA, and London, UK. Furthermore, this survey spanned across European regions from Barcelona, ES, to Bucharest, RO. The joint analysis of all data allows us to focus on general emission behavior for cities with different infrastructure and environmental conditions. We find that all cities have a spectrum of small, medium, and large methane sources in their domain. The emission rates found follow a heavy-tailed distribution, and the top 10% of emitters account for 60-80% of total emissions, which implies that strategic repair planning could help reduce emissions quickly. Furthermore, we compare our findings with inventory estimates for urban natural gas-related methane emissions from this sector in Europe. While cities with larger reported emissions were found to generally also have larger observed emissions, we find clear discrepancies between observation-based and inventory-based emission estimates for our 12 cities.

摘要

为了减少城市天然气配送系统的甲烷排放,了解当地的泄漏率和发生率至关重要。为了探究美国以外城市的城市甲烷排放情况(此前已发现这些城市存在大量排放),在八个国家的12个城市进行了移动测量。被调查的城市规模各异,从中等规模的城市,如荷兰的格罗宁根,到大型城市,如加拿大的多伦多和英国的伦敦。此外,此次调查涵盖了从西班牙巴塞罗那到罗马尼亚布加勒斯特的欧洲地区。对所有数据的联合分析使我们能够关注不同基础设施和环境条件城市的总体排放行为。我们发现,所有城市在其区域内都有一系列小型、中型和大型甲烷源。所发现的排放率遵循重尾分布,前10%的排放源占总排放量的60 - 80%,这意味着战略性的修复计划有助于迅速减少排放。此外,我们将我们的研究结果与欧洲该部门城市天然气相关甲烷排放的清单估计值进行了比较。虽然报告排放量较大的城市通常观测到的排放量也较大,但我们发现我们所研究的12个城市基于观测和基于清单的排放估计之间存在明显差异。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8eee/10851421/3788a00fc88e/es3c03160_0001.jpg

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