Baßler Nico S, Aiello Andrea, Schmidt Kai P, Genes Claudiu, Reitz Michael
Max Planck Institute for the Science of Light, D-91058 Erlangen, Germany.
Department of Physics, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), D-91058 Erlangen, Germany.
Phys Rev Lett. 2024 Jan 26;132(4):043602. doi: 10.1103/PhysRevLett.132.043602.
Quantum metasurfaces, i.e., two-dimensional subwavelength arrays of quantum emitters, can be employed as mirrors towards the design of hybrid cavities, where the optical response is given by the interplay of a cavity-confined field and the surface modes supported by the arrays. We show that stacked layers of quantum metasurfaces with orthogonal dipole orientation can serve as helicity-preserving cavities. These structures exhibit ultranarrow resonances and can enhance the intensity of the incoming field by orders of magnitude, while simultaneously preserving the handedness of the field circulating inside the resonator, as opposed to conventional cavities. The rapid phase shift in the cavity transmission around the resonance can be exploited for the sensitive detection of chiral scatterers passing through the cavity. We discuss possible applications of these resonators as sensors for the discrimination of chiral molecules. Our approach describes a new way of chiral sensing via the measurement of particle-induced phase shifts.
量子超表面,即量子发射器的二维亚波长阵列,可作为设计混合腔的镜子,其中光学响应由腔限制场与阵列支持的表面模式之间的相互作用给出。我们表明,具有正交偶极子取向的量子超表面堆叠层可作为保螺旋度腔。这些结构表现出超窄共振,可将入射场的强度提高几个数量级,同时保持谐振器内循环场的手性,这与传统腔不同。共振附近腔传输中的快速相移可用于灵敏检测穿过腔的手性散射体。我们讨论了这些谐振器作为区分手性分子的传感器的可能应用。我们的方法描述了一种通过测量粒子诱导相移进行手性传感的新方法。