CESAM and Chemistry Department, University of Aveiro, 3810-193, Aveiro, Portugal.
I3N and Department of Physics, University of Aveiro, 3810-193, Aveiro, Portugal.
Anal Bioanal Chem. 2024 Mar;416(8):1983-1995. doi: 10.1007/s00216-024-05199-8. Epub 2024 Feb 15.
Phytotoxins produced by marine microalgae, such as paralytic shellfish toxins (PSTs), can accumulate in bivalve molluscs, representing a human health concern due to the life-threatening symptoms they cause. To avoid the commercialization of contaminated bivalves, monitoring programs were established in the EU. The purpose of this work is the implementation of a PST transforming enzyme-carbamoylase-in an impedimetric test for rapid simultaneous detection of several carbamate and N-sulfocarbamoyl PSTs. Carbamoylase hydrolyses carbamate and sulfocarbamoyl toxins, which may account for up to 90% of bivalve toxicity related to PSTs. Conformational changes of carbamoylase accompanying enzymatic reactions were probed by Fourier transform mid-infrared spectroscopy (FT-MIR) and electrochemical impedance spectroscopy (EIS). Furthermore, a combination of EIS with a metal electrode and a carbamoylase-based assay was employed to harness changes in the enzyme conformation and adsorption on the electrode surface during the enzymatic reaction as an analytical signal. After optimization of the working conditions, the developed impedimetric e-tongue could quantify N-sulfocarbamoyl toxins with a detection limit of 0.1 µM. The developed e-tongue allows the detection of these toxins at concentration levels observed in bivalves with PST toxicity close to the regulatory limit. The quantification of a sum of N-sulfocarbamoyl PSTs in naturally contaminated mussel extracts using the developed impedimetric e-tongue has been demonstrated.
海洋微藻产生的植物毒素,如麻痹性贝类毒素(PSTs),可以在双壳类软体动物中积累,由于它们引起的危及生命的症状,对人类健康构成了威胁。为了避免受污染的双壳类动物的商业化,欧盟建立了监测计划。这项工作的目的是在电化学生物传感器中实现 PST 转化酶-氨甲酰酶的应用,用于快速同时检测几种氨基甲酸酯和 N-磺基氨甲酰 PSTs。氨甲酰酶可水解氨基甲酸酯和磺基氨甲酰毒素,这些毒素可能占与 PST 相关的双壳类动物毒性的 90%。傅里叶变换中红外光谱(FT-MIR)和电化学阻抗谱(EIS)探测到伴随酶反应的氨甲酰酶构象变化。此外,电化学阻抗谱与金属电极和基于氨甲酰酶的测定相结合,利用酶构象在酶反应过程中的变化以及在电极表面的吸附作为分析信号。优化工作条件后,开发的电化学生物传感器可以定量检测 N-磺基氨甲酰毒素,检测限为 0.1µM。该电化学生物传感器可检测 PST 毒性贝类中观察到的接近监管限值的浓度水平的这些毒素。已经证明,使用开发的电化学生物传感器可以定量检测天然污染贻贝提取物中的 N-磺基氨甲酰 PST 总和。