Ki Yu Geun, Jeon Byeong Je, Song Il Hoon, Kim Seong Jun, Jeon Sangtae, Kim Soo Jin
School of Electrical Engineering, Korea University, Seoul 02841, Republic of Korea.
ACS Nano. 2024 Mar 5;18(9):7064-7073. doi: 10.1021/acsnano.3c10749. Epub 2024 Feb 19.
Recent development in nonlocal resonance based chiral metasurfaces draws great attention due to their abilities to strongly interact with circularly polarized light at a relatively narrow spectral bandwidth. However, there still remain challenges in realizing effective nonlocal chiral metasurfaces in optical frequency due to demanding fabrications such as 3D-multilayered or nanoscaled chiral geometry, which, in particular, limit their applications to polarimetric detection with high-Q spectra. Here, we study the underlying working principles and reveal the important role of the interaction between high-Q nonlocal resonance and low-Q localized Mie resonance in realizing effective nonlocal chiral metasurfaces. Based on the working principles, we demonstrate one of the simplest types of nonlocal chiral metasurfaces which directly detects a set of Stokes parameters without the numerical combination of transmitted values presented from typical Stokes metasurfaces. This is achieved by minimally altering the geometry and filling ratio of every constituent nanostructure in a unit cell, facilitating consistent-sized nanolithography for all samples experimentally at a targeted wavelength with relatively high-Q spectra. This work provides an alternative design rule to realizing effective polarimetric metasurfaces and the potential applications of nonlocal Stokes parameters detection.
基于非局域共振的手性超表面的最新进展引起了极大关注,因为它们能够在相对较窄的光谱带宽内与圆偏振光发生强烈相互作用。然而,由于诸如三维多层或纳米级手性几何结构等苛刻的制造要求,在光频中实现有效的非局域手性超表面仍然存在挑战,这尤其限制了它们在具有高Q光谱的偏振检测中的应用。在此,我们研究了其潜在的工作原理,并揭示了高Q非局域共振与低Q局域米氏共振之间的相互作用在实现有效的非局域手性超表面中的重要作用。基于这些工作原理,我们展示了一种最简单的非局域手性超表面类型,它可以直接检测一组斯托克斯参数,而无需对典型斯托克斯超表面给出的透射值进行数值组合。这是通过最小化改变晶胞中每个组成纳米结构的几何形状和填充率来实现的,便于在实验中以相对高Q光谱在目标波长下对所有样品进行尺寸一致的纳米光刻。这项工作为实现有效的偏振超表面提供了一种替代设计规则以及非局域斯托克斯参数检测的潜在应用。