Ji Xinyi, Fan Xiangqian, Liu Xue, Gu Jianfeng, Lu Haolin, Luan Zhaohui, Liang Jiajie
School of Materials Science and Engineering, Nankai University, Tianjin 300350, P. R. China.
School of Energy and Power Engineering, North University of China, Taiyuan 030051, P. R. China.
Nano Lett. 2024 Mar 20;24(11):3498-3506. doi: 10.1021/acs.nanolett.4c00456. Epub 2024 Mar 5.
Solar distillation is a promising approach for addressing water scarcity, but relentless stress/strain perturbations induced by wind and waves would inevitably cause structural damage to solar absorbers. Despite notable advances in efficient solar absorbers, there have been no reports of compliant and robust solar absorbers withstanding practical mechanical impacts. Herein, an elastic and robust hydrogel absorber that exhibited a high level of evaporation performance was fabricated by introducing ion-coordinated MXene nanosheets as photothermal conversion units and mechanically enhanced fillers. The ion-coordinated MXene nanosheets acting as strong cross-linking points provided excellent elasticity and robustness to the hydrogel absorber. As a result, the evaporation rate of hydrogel absorber, with a high initial value of 2.61 kg m h under one sun irradiation, remained at 2.15 kg m h under a 100% tensile strain state and 2.40 kg m h after 10 000 stretching-releasing cycles. This continuous and stable water desalination approach provides a promising device for actual seawater distillation.
太阳能蒸馏是解决水资源短缺问题的一种很有前景的方法,但风浪引起的持续应力/应变扰动不可避免地会对太阳能吸收器造成结构损坏。尽管高效太阳能吸收器取得了显著进展,但尚无关于能承受实际机械冲击的柔顺且坚固的太阳能吸收器的报道。在此,通过引入离子配位的MXene纳米片作为光热转换单元和机械增强填料,制备了一种具有高蒸发性能的弹性且坚固的水凝胶吸收器。作为强交联点的离子配位MXene纳米片赋予了水凝胶吸收器优异的弹性和坚固性。结果,水凝胶吸收器在一个太阳辐照下的初始蒸发速率高达2.61 kg m⁻² h⁻¹,在100%拉伸应变状态下保持在2.15 kg m⁻² h⁻¹,经过10000次拉伸-释放循环后仍为2.40 kg m⁻² h⁻¹。这种连续稳定的海水淡化方法为实际的海水蒸馏提供了一种很有前景的装置。