Liu Pan, Hu Yi-Bo, Li Xiao-Ying, Xu Lei, Chen Chen, Yuan Baoling, Fu Ming-Lai
Xiamen Key Laboratory of Municipal and Industrial Solid Waste Utilization and Pollution Control, College of Civil Engineering, Huaqiao University, Xiamen, Fujian 361021, P. R. China.
Key Laboratory of Songliao Aquatic Environment, Ministry of Education, Jilin Jianzhu University, Changchun, 130118, P. R. China.
Angew Chem Int Ed Engl. 2022 Sep 12;61(37):e202208587. doi: 10.1002/anie.202208587. Epub 2022 Jul 19.
Interfacial photo-vapor conversion has been suggested as a cost-effective and sustainable technology for seawater desalination. However, the conversion performance was still limited by some drawbacks, like salt accumulation and poor mechanical stability. Herein, a scalable MoS -based porous hydrogel (SMoS -PH) with good mechanical stability and salt resistance was successfully constructed through a crosslinking foaming polymerization method. With the high porosity (92.63 %), the SMoS -PH performed an impressive evaporation rate of 3.297 kg m h and photothermal conversion efficiency of 93.4 % under 1-sun illumination. Most importantly, the SMoS -PH could maintain high and stable photothermal properties for 15 days on the surface of seawater. We believe that the excellent salt resistance, the high photothermal conversion efficiency, the ease of scale preparation method and the available commercial MoS make the SMoS -PH a promising device for full-scale seawater desalination.
界面光蒸汽转换被认为是一种用于海水淡化的具有成本效益且可持续的技术。然而,转换性能仍受到一些缺点的限制,如盐分积累和机械稳定性差。在此,通过交联发泡聚合法成功构建了一种具有良好机械稳定性和耐盐性的可扩展的基于MoS的多孔水凝胶(SMoS-PH)。具有92.63%的高孔隙率,SMoS-PH在1个太阳光照下表现出令人印象深刻的3.297 kg m² h的蒸发速率和93.4%的光热转换效率。最重要的是,SMoS-PH在海水表面可保持15天的高稳定光热性能。我们相信,优异的耐盐性、高光热转换效率、易于规模化制备的方法以及可得的商业MoS使SMoS-PH成为一种有前景的大规模海水淡化装置。