Zhou Weijian, Ma Tieying, Tian Ye, Jiang Yixin, Yu Xuechao
College of Optical and Electronic Technology, China Jiliang University, Hangzhou 310013, China.
Key Laboratory of Multifunctional Nanomaterials and Smart Systems, Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences, Suzhou, Jiangsu 215123, China.
iScience. 2024 Feb 23;27(3):109314. doi: 10.1016/j.isci.2024.109314. eCollection 2024 Mar 15.
Graphene, known for its ultrahigh carrier mobility and broadband optical absorption, holds significant potential in optoelectronics. However, the carrier mobility of graphene on silicon substrates experienced a marked decrease due to surface roughness, phonon scattering affects. Here we report carrier mobility enhancement of graphene dielectric engineering. Through the fabrication of devices utilizing Si/SiO/AlO/graphene layers and subsequent electrical characterization, our findings illustrate the navigable nature of the AlO dielectric layer is navigable for reducing the SiO phonon scattering and increasing graphene's carrier mobility by up to ∼8000 cmVs. Furthermore, the improvement in carrier mobility of graphene has been utilized in the hybrid near-infrared photodetector, resulting in outstanding responsivity of ∼400 AW, detectivity of ∼2.2 ✕ 10 Jones in the graphene/AgTe detector. Our study establishes pathways for the seamless integration of graphene or other 2D materials within the standard CMOS processes, thereby facilitating the fabrication of advanced optoelectronic devices.
石墨烯以其超高的载流子迁移率和宽带光吸收而闻名,在光电子学领域具有巨大潜力。然而,由于表面粗糙度和声子散射的影响,硅衬底上石墨烯的载流子迁移率显著下降。在此,我们报告了通过介电工程提高石墨烯的载流子迁移率。通过制备使用Si/SiO/AlO/石墨烯层的器件并进行后续电学表征,我们的研究结果表明,AlO介电层对于减少SiO声子散射和将石墨烯的载流子迁移率提高至约8000 cm²V⁻¹s⁻¹具有可操作性。此外,石墨烯载流子迁移率的提高已应用于混合近红外光电探测器,在石墨烯/AgTe探测器中产生了约400 A/W的出色响应度和约2.2×10¹² Jones的探测率。我们的研究为石墨烯或其他二维材料在标准CMOS工艺中的无缝集成开辟了道路,从而促进了先进光电器件的制造。