Yan Jin, Kong Haoran, Li Yuting, Wang Qinhuan, Liu Xiang, Wang Yu
State Key Laboratory of Mesoscience and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, People's Republic of China.
School of Chemical Engineering, University of Chinese Academy of Sciences, Beijing 100049, People's Republic of China.
Nano Lett. 2024 Mar 20;24(11):3515-3524. doi: 10.1021/acs.nanolett.4c00487. Epub 2024 Mar 8.
As a promising fresh water harvesting technology, interfacial solar steam generation has attracted growing interest. Efficient solar absorption and long-term operational performance are critical requirements of this technology. However, developing robust evaporators to promote practical applications under extreme conditions is still a grand challenge. Herein, we propose a light-assisted strategy to in situ prepare a TiCT MXene anchored structure (MXAS) for enhanced solar evaporation with superior mechanical properties (compressive strength of 78.47 MPa, which can withstand a pressure of 3.92 × 10 times its own weight). Light irradiation enlarges the interlayer spacing of MXene and improves the solar absorption capability. Under one sun, the three-dimensional MXAS evaporator exhibits a steam generation rate of 2.48 kg m hand an evaporation efficiency of 89.3%, and it demonstrates long-term durability when testing in seawater. This strategy provides valuable insights into the potential application of a high-performance water evaporation system.
作为一种很有前景的淡水收集技术,界面太阳能蒸汽产生已引起越来越多的关注。高效的太阳能吸收和长期的运行性能是该技术的关键要求。然而,开发坚固的蒸发器以促进其在极端条件下的实际应用仍然是一个巨大的挑战。在此,我们提出一种光辅助策略,原位制备一种TiCT MXene锚定结构(MXAS),以增强太阳能蒸发,同时具有优异的机械性能(抗压强度为78.47 MPa,可承受自身重量3.92×10倍的压力)。光辐照增大了MXene的层间距,提高了太阳能吸收能力。在一个太阳光照强度下,三维MXAS蒸发器的蒸汽产生速率为2.48 kg m² h,蒸发效率为89.3%,并且在海水中测试时表现出长期耐久性。该策略为高性能水蒸发系统的潜在应用提供了有价值的见解。