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CrSBr:一种空气稳定的二维磁性半导体。

CrSBr: An Air-Stable, Two-Dimensional Magnetic Semiconductor.

作者信息

Ziebel Michael E, Feuer Margalit L, Cox Jordan, Zhu Xiaoyang, Dean Cory R, Roy Xavier

机构信息

Columbia University, Department of Chemistry, New York, New York 10027, United States.

Columbia University, Department of Physics, New York, New York 10027, United States.

出版信息

Nano Lett. 2024 Apr 17;24(15):4319-4329. doi: 10.1021/acs.nanolett.4c00624. Epub 2024 Apr 3.

Abstract

The discovery of magnetic order at the 2D limit has sparked new exploration of van der Waals magnets for potential use in spintronics, magnonics, and quantum information applications. However, many of these materials feature low magnetic ordering temperatures and poor air stability, limiting their fabrication into practical devices. In this Mini-Review, we present a promising material for fundamental studies and functional use: CrSBr, an air-stable, two-dimensional magnetic semiconductor. Our discussion highlights experimental research on bulk CrSBr, including quasi-1D semiconducting properties, A-type antiferromagnetic order ( = 132 K), and strong coupling between its electronic and magnetic properties. We then discuss the behavior of monolayer and few-layer flakes and present a perspective on promising avenues for further studies on CrSBr.

摘要

二维极限下磁序的发现引发了对范德华磁体的新探索,有望用于自旋电子学、磁子学和量子信息应用。然而,这些材料中的许多都具有较低的磁序温度和较差的空气稳定性,限制了它们制造成实际器件。在本综述中,我们介绍了一种用于基础研究和功能应用的有前景的材料:CrSBr,一种空气稳定的二维磁性半导体。我们的讨论重点介绍了对块状CrSBr的实验研究,包括准一维半导体特性、A型反铁磁序( = 132 K)以及其电子和磁性之间的强耦合。然后,我们讨论了单层和少层薄片的行为,并对CrSBr进一步研究的有前景的途径提出了展望。

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