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考虑磁场和偏振情况下高强度激光脉冲与氢原子相互作用的量子力学建模。

Quantum mechanical modeling of high-intensity laser pulse interaction with hydrogen atom with considering the magnetic field and polarization.

作者信息

Zakavi Marjan, Sabaeian Mohammad

机构信息

Department of Physics, Faculty of Science, Shahid Chamran University of Ahvaz, Ahvaz, Iran.

Center for Research on Laser and Plasma, Shahid Chamran University of Ahvaz, Ahvaz, Iran.

出版信息

Sci Rep. 2024 Apr 18;14(1):9005. doi: 10.1038/s41598-024-59515-4.

Abstract

In the study of the non-relativistic interaction between high-intensity femtosecond laser pulses and atoms, the influence of the magnetic field is commonly overlooked. This work investigates the effects of the magnetic field in the high-intensity few-cycle laser pulses with non-relativistic intensity of at the center wavelength of 800 nm on the high-order harmonic generation (HHG), attosecond pulse train (APT), isolated attosecond pulse (IAP), and the electron trajectory in the hydrogen atom, employing the numerical solution of the time-dependent Schrödinger equation in three dimensions (3D-TDSE). Two polarizations, linear and circular, are considered. A comparison with the scenario where the magnetic field is not considered shows that the magnetic field can apply significant corrections to the results. Particularly, considering the magnetic field for circular polarization can make the cutoff frequency of HHG coincide with the semi-classical relationship of , a case that for circular polarization does not exist without considering the magnetic field. Moreover, accounting for the magnetic field leads to a reduction in the attosecond pulse duration for circular polarization for APT ( versus ) and for IAP ( versus ). Additionally, the difference in production efficiency of HHG and APT between linear and circular polarization is reduced by two orders of magnitude, when magnetic field is considered. Although considering the magnetic field complicates the electron trajectory, especially for circular polarization, however, our quantum model provides enhanced insight into how the interaction works, especially when and where the electron collides with the parent nucleus. In this case, the quantum mechanical modeling largely covers the huge difference of not considering the magnetic field in the results predicted by other works.

摘要

在高强度飞秒激光脉冲与原子之间的非相对论相互作用研究中,磁场的影响通常被忽视。本工作利用三维含时薛定谔方程(3D - TDSE)的数值解,研究了中心波长为800 nm、非相对论强度的高强度少周期激光脉冲中的磁场对高次谐波产生(HHG)、阿秒脉冲串(APT)、孤立阿秒脉冲(IAP)以及氢原子中电子轨迹的影响。考虑了线性和圆偏振两种偏振情况。与不考虑磁场的情况相比表明,磁场可以对结果进行显著修正。特别地,对于圆偏振考虑磁场可使HHG的截止频率与半经典关系 相符,而在不考虑磁场的情况下,圆偏振不存在这种情况。此外,考虑磁场会导致APT的圆偏振阿秒脉冲持续时间缩短( 对比 )以及IAP的圆偏振阿秒脉冲持续时间缩短( 对比 )。另外,当考虑磁场时,线性偏振和圆偏振之间HHG和APT产生效率的差异降低了两个数量级。尽管考虑磁场会使电子轨迹变得复杂,尤其是对于圆偏振,但我们的量子模型能更深入地洞察相互作用的工作方式,特别是电子与母核碰撞的时间和位置。在这种情况下,量子力学建模在很大程度上弥补了其他工作预测结果中不考虑磁场时的巨大差异。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7992/11551220/37c20b63053b/41598_2024_59515_Fig1_HTML.jpg

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