Kee Jung Yun, Kim Kook Tae, Lee In Hak, Seo Ilwan, Chang Jun-Young, Lee Ah-Yeon, Noh Woo-Suk, Chang Young Jun, Park Seung-Young, Choe Sug-Bong, Kim Duck-Ho, Kim Kyoung-Whan, Choi Yongseong, Lee Dong Ryeol, Choi Jun Woo
Center for Spintronics, Korea Institute of Science and Technology (KIST), Seoul, 02792, Korea.
Department of Physics, Soongsil University, Seoul, 06978, Korea.
Sci Rep. 2024 Apr 25;14(1):9476. doi: 10.1038/s41598-024-60076-9.
Interfacial magnetic interactions between different elements are the origin of various spin-transport phenomena in multi-elemental magnetic systems. We investigate the coupling between the magnetic moments of the rare-earth, transition-metal, and heavy-metal elements across the interface in a GdFeCo/Pt thin film, an archetype system to investigate ferrimagnetic spintronics. The Pt magnetic moments induced by the antiferromagnetically aligned FeCo and Gd moments are measured using element-resolved x-ray measurements. It is revealed that the proximity-induced Pt magnetic moments are always aligned parallel to the FeCo magnetic moments, even below the ferrimagnetic compensation temperature where FeCo has a smaller moment than Gd. This is understood by a theoretical model showing distinct effects of the rare-earth Gd 4f and transition-metal FeCo 3d magnetic moments on the Pt electronic states. In particular, the Gd and FeCo work in-phase to align the Pt moment in the same direction, despite their antiferromagnetic configuration. The unexpected additive roles of the two antiferromagnetically coupled elements exemplify the importance of detailed interactions among the constituent elements in understanding magnetic and spintronic properties of thin film systems.
不同元素之间的界面磁相互作用是多元素磁系统中各种自旋输运现象的起源。我们研究了GdFeCo/Pt薄膜(一种用于研究亚铁磁自旋电子学的典型系统)中稀土、过渡金属和重金属元素的磁矩在界面处的耦合。利用元素分辨x射线测量方法测量了由反铁磁排列的FeCo和Gd磁矩诱导的Pt磁矩。结果表明,即使在亚铁磁补偿温度以下(此时FeCo的磁矩小于Gd),邻近诱导的Pt磁矩也总是与FeCo磁矩平行排列。这可以通过一个理论模型来理解,该模型表明稀土Gd 4f和过渡金属FeCo 3d磁矩对Pt电子态有不同的影响。特别是,尽管Gd和FeCo呈反铁磁构型,但它们协同作用使Pt磁矩沿相同方向排列。这两个反铁磁耦合元素出人意料的相加作用体现了组成元素之间详细相互作用在理解薄膜系统的磁性和自旋电子学性质方面的重要性。