Céspedes-Berrocal David, Damas Heloïse, Petit-Watelot Sébastien, Maccariello Davide, Tang Ping, Arriola-Córdova Aldo, Vallobra Pierre, Xu Yong, Bello Jean-Loïs, Martin Elodie, Migot Sylvie, Ghanbaja Jaafar, Zhang Shufeng, Hehn Michel, Mangin Stéphane, Panagopoulos Christos, Cros Vincent, Fert Albert, Rojas-Sánchez Juan-Carlos
Institute Jean Lamour, Université de Lorraine, CNRS, Nancy, F-54000, France.
Facultad de Ciencias, Universidad Nacional de Ingeniería, Rímac, Lima, 15333, Peru.
Adv Mater. 2021 Mar;33(12):e2007047. doi: 10.1002/adma.202007047. Epub 2021 Feb 19.
Spintronics exploit spin-orbit coupling (SOC) to generate spin currents, spin torques, and, in the absence of inversion symmetry, Rashba and Dzyaloshinskii-Moriya interactions. The widely used magnetic materials, based on 3d metals such as Fe and Co, possess a small SOC. To circumvent this shortcoming, the common practice has been to utilize the large SOC of nonmagnetic layers of 5d heavy metals (HMs), such as Pt, to generate spin currents and, in turn, exert spin torques on the magnetic layers. Here, a new class of material architectures is introduced, excluding nonmagnetic 5d HMs, for high-performance spintronics operations. Very strong current-induced torques exerted on single ferrimagnetic GdFeCo layers, due to the combination of large SOC of the Gd 5d states and inversion symmetry breaking mainly engineered by interfaces, are demonstrated. These "self-torques" are enhanced around the magnetization compensation temperature and can be tuned by adjusting the spin absorption outside the GdFeCo layer. In other measurements, the very large emission of spin current from GdFeCo, 80% (20%) of spin anomalous Hall effect (spin Hall effect) symmetry is determined. This material platform opens new perspectives to exert "self-torques" on single magnetic layers as well as to generate spin currents from a magnetic layer.
自旋电子学利用自旋轨道耦合(SOC)来产生自旋电流、自旋扭矩,并且在不存在空间反演对称性的情况下,还能产生Rashba和Dzyaloshinskii-Moriya相互作用。广泛使用的基于铁和钴等3d金属的磁性材料,其SOC较小。为了克服这一缺点,常见的做法是利用5d重金属(HMs)的非磁性层(如铂)的大SOC来产生自旋电流,进而对磁性层施加自旋扭矩。在此,引入了一类新型的材料结构,不包括非磁性5d HMs,用于高性能自旋电子学操作。通过实验证明,由于Gd 5d态的大SOC与主要由界面设计的空间反演对称性破缺相结合,在单个亚铁磁性GdFeCo层上施加了非常强的电流诱导扭矩。这些“自扭矩”在磁化补偿温度附近增强,并且可以通过调节GdFeCo层外的自旋吸收来调整。在其他测量中,确定了GdFeCo的自旋电流发射非常大,自旋反常霍尔效应(自旋霍尔效应)对称性的80%(20%)。这个材料平台为在单个磁性层上施加“自扭矩”以及从磁性层产生自旋电流开辟了新的前景。