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拓扑谷霍尔极化激元凝聚

Topological valley Hall polariton condensation.

作者信息

Peng Kai, Li Wei, Sun Meng, Rivero Jose D H, Ti Chaoyang, Han Xu, Ge Li, Yang Lan, Zhang Xiang, Bao Wei

机构信息

Department of Materials Science and Engineering, Rensselaer Polytechnic Institute, Troy, NY, USA.

Nanoscale Science and Engineering Center, University of California, Berkeley, Berkeley, CA, USA.

出版信息

Nat Nanotechnol. 2024 Sep;19(9):1283-1289. doi: 10.1038/s41565-024-01674-6. Epub 2024 May 24.

Abstract

A photonic topological insulator features robust directional propagation and immunity to defect perturbations of the edge/surface state. Exciton-polaritons, that is, the hybrid quasiparticles of excitons and photons in semiconductor microcavities, have been proposed as a tunable nonlinear platform for emulating topological phenomena. However, mainly due to excitonic material limitations, experimental observations so far have not been able to enter the nonlinear condensation regime or only show localized condensation in one dimension. Here we show a topological propagating edge state with polariton condensation at room temperature and without any external magnetic field. We overcome material limitations by using excitonic CsPbCl halide perovskites with a valley Hall lattice design. The polariton lattice features a large bandgap of 18.8 meV and exhibits strong nonlinear polariton condensation with clear long-range spatial coherence across the critical pumping density. The geometric parameters and material composition of our nonlinear many-body photonic system platform can in principle be tailored to study topological phenomena of other interquasiparticle interactions.

摘要

光子拓扑绝缘体具有稳健的定向传播特性,且其边缘/表面态对缺陷微扰具有免疫能力。激子极化激元,即半导体微腔中激子与光子的混合准粒子,已被提议作为一种用于模拟拓扑现象的可调谐非线性平台。然而,主要由于激子材料的局限性,迄今为止的实验观测尚未能够进入非线性凝聚 regime,或者仅在一维中表现出局域凝聚。在此,我们展示了一种在室温下且无需任何外部磁场的情况下具有极化激元凝聚的拓扑传播边缘态。我们通过使用具有谷霍尔晶格设计的激子型 CsPbCl 卤化物钙钛矿克服了材料局限性。该极化激元晶格具有 18.8 meV 的大带隙,并在临界泵浦密度下展现出具有清晰长程空间相干性的强非线性极化激元凝聚。我们的非线性多体光子系统平台的几何参数和材料组成原则上可以进行定制,以研究其他准粒子间相互作用的拓扑现象。

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