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室温下钙钛矿莫尔平带中的激子极化激元凝聚

Exciton polariton condensation in a perovskite moiré flat band at room temperature.

作者信息

Jin Feng, Ren Jiahao, Zanotti Simone, Cui Peiyuan, Zheng Hao, Liang Jie, Ni Jinyang, Wang Zhe, Shi Fulong, Qiu Cheng-Wei, Chang Guoqing, Liew Timothy C H, Su Rui

机构信息

Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore.

Department of Electrical and Computer Engineering, National University of Singapore, Singapore 117583, Singapore.

出版信息

Sci Adv. 2025 Aug 8;11(32):eadx2361. doi: 10.1126/sciadv.adx2361. Epub 2025 Aug 6.

Abstract

Moiré superlattices exhibit fascinating moiré flat bands when two layers of van der Waals materials are twisted at specific magic angles, providing unparalleled opportunities to explore unconventional correlated quantum phenomena. Exciton polaritons, hybrid quasiparticles of excitons and photons, have emerged as promising synthetic platforms for exploring moiré physics beyond conventional systems. However, the realization of moiré exciton-polariton flat bands and their condensation remains challenging. Here, we experimentally demonstrate a moiré exciton-polariton flat band with condensation in a perovskite moiré superlattice at room temperature. By engineering a 21.79° magic-angle moiré superlattice potential with enhanced interlayer coupling, we experimentally observe a polaritonic moiré flat band near the corresponding monolayer's Dirac points position in the perovskite microcavity. Under a nonresonant pulsed excitation, polaritons with proper detuning condense into the moiré flat band at room temperature. Our work provides a unique platform for investigating exotic moiré phenomena and unlocks promising avenues toward advanced polaritonic devices.

摘要

当两层范德华材料以特定的神奇角度扭曲时,莫尔超晶格会展现出迷人的莫尔平带,为探索非常规关联量子现象提供了无与伦比的机会。激子极化激元是激子和光子的混合准粒子,已成为探索超越传统系统的莫尔物理的有前景的合成平台。然而,实现莫尔激子 - 极化激元平带及其凝聚仍然具有挑战性。在此,我们通过实验证明了在室温下钙钛矿莫尔超晶格中具有凝聚现象的莫尔激子 - 极化激元平带。通过设计具有增强层间耦合的21.79°神奇角度莫尔超晶格势,我们在钙钛矿微腔中相应单层狄拉克点位置附近实验观察到极化激元莫尔平带。在非共振脉冲激发下,具有适当失谐的极化激元在室温下凝聚到莫尔平带中。我们的工作为研究奇异的莫尔现象提供了一个独特的平台,并为先进的极化激元器件开辟了有前景的途径。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b045/12327445/bbccb31c90c0/sciadv.adx2361-f1.jpg

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