Chen Jia-Yin, Huang Kang-Ting, Yau Shuehlin, Huang Chun-Jen
Department of Chemical & Materials Engineering, National Central University, Jhong-Li, Taoyuan 320, Taiwan.
R&D Center for Membrane Technology, Chung Yuan Christian University, 200 Chung Pei Rd., Chung-Li City 32023, Taiwan.
Langmuir. 2024 Jun 25;40(25):13236-13246. doi: 10.1021/acs.langmuir.4c01395. Epub 2024 Jun 12.
A biocompatible and antifouling polymeric medical coating was developed through rational design for anchoring pendant groups for the modification of stainless steel. Zwitterionic 2-methacryloyloxyethyl phosphorylcholine (MPC) was copolymerized individually with three anchoring monomers of carboxyl acrylamides with different alkyl spacers, including acryloylglycine (2-AE), 6-acrylamidohexanoic acid (6-AH), and 11-acrylamidoundecanoic acid (11-AU). The carboxylic acid groups are responsible for the stable grafting of copolymers onto stainless steel via a coordinative interaction with metal oxides. Due to hydrophobic interaction and hydrogen bonding, the anchoring monomers enable the formation of self-assembling structures in solution and at a metallic interface, which can play an important role in the thin film formation and functionality of the coatings. Therefore, surface characterizations of anchoring monomers on stainless steel were conducted to analyze the packing density and strength of the intermolecular hydrogen bonds. The corresponding copolymers were synthesized, and their aggregate structures were assessed, showing micelle aggregation for copolymers with higher hydrophobic compositions. The synergistic effects of inter/intramolecular interactions and hydrophobicity of the anchoring monomers result in the diversity of the thickness, surface coverage, wettability, and friction of the polymeric coatings on stainless steel. More importantly, the antifouling properties of the coatings against bacteria and proteins were strongly correlated to thin film formation. Ultimately, the key lies in deciphering the molecular structure of the anchoring pendants in thin film formation and assessing the effectiveness of the coatings, which led to the development of medical coatings through the graft-onto approach.
通过合理设计用于锚固侧基以修饰不锈钢,开发了一种具有生物相容性和抗污性的聚合物医用涂层。两性离子型2-甲基丙烯酰氧基乙基磷酰胆碱(MPC)分别与三种具有不同烷基间隔基的羧基丙烯酰胺锚固单体共聚,包括丙烯酰甘氨酸(2-AE)、6-丙烯酰胺基己酸(6-AH)和11-丙烯酰胺基十一酸(11-AU)。羧酸基团通过与金属氧化物的配位相互作用负责将共聚物稳定接枝到不锈钢上。由于疏水相互作用和氢键作用,锚固单体能够在溶液中和金属界面形成自组装结构,这在涂层的薄膜形成和功能中可以发挥重要作用。因此,对不锈钢上的锚固单体进行了表面表征,以分析分子间氢键的堆积密度和强度。合成了相应的共聚物,并评估了它们的聚集结构,结果表明具有较高疏水组成的共聚物形成胶束聚集。锚固单体的分子间/分子内相互作用和疏水性的协同作用导致了不锈钢上聚合物涂层在厚度、表面覆盖率、润湿性和摩擦方面的多样性。更重要的是,涂层对细菌和蛋白质的抗污性能与薄膜形成密切相关。最终,关键在于破译薄膜形成中锚固侧基的分子结构并评估涂层的有效性,这导致了通过接枝法开发医用涂层。