Carvalho William O F, Spadoti Danilo H, Oliveira Osvaldo N, Mejía-Salazar Jorge Ricardo
Sao Carlos Institute of Physics, University of Sao Paulo, CP 369, 13560-970 São Carlos, São Paulo, Brazil.
Federal University of Itajubá (UNIFEI), 37500-903 Itajubá, Minas Gerais, Brazil.
ACS Appl Mater Interfaces. 2024 Aug 14;16(32):42942-42946. doi: 10.1021/acsami.4c08601. Epub 2024 Aug 1.
Conventional magnetophotonic nanostructures typically function within narrow wavelength and incident angle ranges, where resonance is observed and magneto-optical (MO) effects are amplified. Expanding these operational ranges may allow for improved applications, including in (bio)sensing devices. In this study, we describe a hybrid magnetoplasmonic waveguide grating (HMPWG) in which the coupling of plasmonic resonances and waveguide modes leads to enhanced MO effects and sensitivity, according to full-wave electromagnetic simulations. High transverse magneto-optical Kerr effect (TMOKE) signals were observed for the full range of wavelengths and angles investigated, i.e., for θ ≥ 1° and 500 nm ≤ λ ≤ 850 nm. As a proof-of-concept we verified that using the HMPWG nanostructure with an aqueous solution as superstrate one may obtain a sensitivity in variation of the refractive index unit (RIU) of = 166°/RIU and = 230 nm/RIU in angle and wavelength interrogation modes, respectively. Upon comparing with conventional magnetoplasmonic gratings, which only enable excitation of plasmonic resonances, we demonstrate that HMPWG nanostructures can be further optimized to reach not only high sensitivity but also high resolution in sensing and biosensing.
传统的磁光光子纳米结构通常在窄波长和入射角范围内起作用,在该范围内会观察到共振且磁光(MO)效应会被放大。扩大这些工作范围可能会改进应用,包括在(生物)传感设备中的应用。在本研究中,我们描述了一种混合磁等离子体波导光栅(HMPWG),根据全波电磁模拟,其中等离子体共振与波导模式的耦合会导致增强的MO效应和灵敏度。在所研究的整个波长和角度范围内,即对于θ≥1°且500nm≤λ≤850nm,均观察到了高横向磁光克尔效应(TMOKE)信号。作为概念验证,我们证实,使用以水溶液为上层介质的HMPWG纳米结构,在角度和波长询问模式下,折射率单位(RIU)变化的灵敏度分别为 = 166°/RIU和 = 230nm/RIU。与仅能激发等离子体共振的传统磁等离子体光栅相比,我们证明HMPWG纳米结构不仅可以进一步优化以实现高灵敏度,还能在传感和生物传感中实现高分辨率。