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悬浮微滴簇中化学反应的观察及液滴生成的音乐。

Observation of a chemical reaction in a levitating microdroplet cluster and droplet-generated music.

作者信息

Fedorets Alexander A, Koltsov Semyon, Muravev Anton A, Fotin Alexey, Zun Pavel, Orekhov Nikita, Nosonovsky Michael, Skorb Ekaterina V

机构信息

X-BIO Institute, University of Tyumen Tyumen 625003 Russia.

ITMO University St. Petersburg 191002 Russia

出版信息

Chem Sci. 2024 Jun 27;15(30):12067-12076. doi: 10.1039/d4sc03066d. eCollection 2024 Jul 31.

DOI:10.1039/d4sc03066d
PMID:39092132
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11290446/
Abstract

Ordered clusters of water droplets levitating over a heated water surface can be used as chemical microreactors and computational devices. Here we show that a chemical reaction between melamine and cyanuric acid can occur during coalescence of pairs of droplets containing these reagents and lead to the sedimentation of the product, crystals of melamine cyanurate. In rotating droplets, the crystals flash with frequencies dependent mostly on the rotational velocity of the droplets defined by the rotor of the velocity field of the air-vapor flow above the heated water surface. With the Machine Learning (ML) approach, we trace the brightness and frequencies of individual crystals and convert the frequencies into musical notes thus making a "micro-orchestra" of the levitation cluster.

摘要

悬浮在热水表面上有序排列的水滴簇可被用作化学微反应器和计算设备。在此我们表明,三聚氰胺和氰尿酸之间的化学反应可在含有这些试剂的液滴对合并过程中发生,并导致产物三聚氰胺氰尿酸晶体的沉淀。在旋转的液滴中,晶体闪烁的频率主要取决于由热水表面上方空气 - 蒸汽流速度场的转子所定义的液滴旋转速度。通过机器学习(ML)方法,我们追踪单个晶体的亮度和频率,并将频率转换为音符,从而制作出悬浮簇的“微型管弦乐队”。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/9d2bfb3110c9/d4sc03066d-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/e7504681dace/d4sc03066d-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/69c51861d61b/d4sc03066d-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/d8a829c2714b/d4sc03066d-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/f5f4d2a97661/d4sc03066d-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/9d2bfb3110c9/d4sc03066d-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/e7504681dace/d4sc03066d-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/69c51861d61b/d4sc03066d-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/d8a829c2714b/d4sc03066d-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/f5f4d2a97661/d4sc03066d-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6777/11290446/9d2bfb3110c9/d4sc03066d-f5.jpg

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本文引用的文献

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Programmable self-organization of heterogeneous microrobot collectives.可编程的异质微型机器人集体自组织。
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Symmetry of small clusters of levitating water droplets.悬浮小水滴簇的对称性。
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Self-Arranged Levitating Droplet Clusters: A Reversible Transition from Hexagonal to Chain Structure.自排列悬浮液滴簇:从六边形到链状结构的可逆转变
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