Castillo López de Larrinzar Beatriz, García Jorge M, Lanzillotti-Kimura Norberto Daniel, García-Martín Antonio
Instituto de Micro y Nanotecnología IMN-CNM, CSIC, CEI UAM+CSIC, Isaac Newton 8, Tres Cantos, 28760 Madrid, Spain.
Centre de Nanosciences et de Nanotechnologies, CNRS, Université Paris-Saclay, 91120 Palaiseau, France.
Nanomaterials (Basel). 2024 Jul 29;14(15):1276. doi: 10.3390/nano14151276.
Non-conventional resonances, both acoustic and photonic, are found in metallic particles with a toroidal nanopropeller geometry, which is generated by sweeping a three-lobed 2D shape along a spiral with twisting angle α. For both optical and acoustic cases, the spectral location of resonances experiences a red-shift as a function of α. We demonstrate that the optical case can be understood as a natural evolution of resonances as the spiral length of the toroidal nanopropeller increases with α, implying a huge helicity-dependent absorption cross-section. In the case of acoustic response, two red-shifting breathing modes are identified. Additionally, even a small α allows the appearance of new low-frequency resonances, whose spectral dispersion depends on a competition between the length of the generative spiral and the pitch of the toroidal nanopropeller.
在具有环形纳米螺旋桨几何形状的金属颗粒中发现了非常规共振,包括声学共振和光子共振,这种几何形状是通过将三叶二维形状沿具有扭转角α的螺旋线扫掠而产生的。对于光学和声学情况,共振的光谱位置都会随着α发生红移。我们证明,随着环形纳米螺旋桨的螺旋长度随α增加,光学情况可被理解为共振的自然演化,这意味着存在巨大的与螺旋度相关的吸收截面。在声学响应的情况下,识别出了两种红移呼吸模式。此外,即使α很小也会出现新的低频共振,其光谱色散取决于生成螺旋线的长度与环形纳米螺旋桨的螺距之间的竞争。