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用于红外光捕获的简并掺杂金属氧化物纳米晶体：对其等离子体特性及未来前景的洞察

Degenerately doped metal oxide nanocrystals for infrared light harvesting: insight into their plasmonic properties and future perspectives.

作者信息

Singh Mandeep, Scotognella Francesco, Paternò Giuseppe Maria

机构信息

Physics Department, Politecnico di Milano Piazza L. da Vinci 32 20133 Milano Italy

Department of Applied Science and Technology, Politecnico di Torino Corso Duca degli Abruzzi 24 Torino 10129 Italy

出版信息

Mater Adv. 2024 Aug 1;5(17):6796-6812. doi: 10.1039/d4ma00426d. eCollection 2024 Aug 27.

DOI:10.1039/d4ma00426d
PMID:39130726
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11307255/
Abstract

The tuneability of the localized surface plasmon resonance (LSPR) of degenerately doped metal oxide (MOX) nanocrystals (NCs) over a wide range of the infrared (IR) region by controlling NC size and doping content offers a unique opportunity to develop a future generation of optoelectronic and photonic devices like IR photodetectors and sensors. The central aim of this review article is to highlight the distinctive and remarkable plasmonic properties of degenerately or heavily doped MOX nanocrystals by reviewing the comprehensive literature reported so far. In particular, the literature of each MOX NC, ZnO, CdO, InO, and WO doped with different dopants, is discussed separately. In addition to discussion of the most commonly used colloidal synthesis approaches, the ultrafast dynamics of charge carriers in NCs and the extraction of LSPR-assisted hot-carriers are also discussed in detail. Finally, future prospective applications of MOX NCs in IR photodetectors and photovoltaic (PV) self-powered chemical sensors are also presented.

摘要

通过控制纳米晶体（NCs）的尺寸和掺杂含量，简并掺杂金属氧化物（MOX）纳米晶体的局域表面等离子体共振（LSPR）在很宽的红外（IR）区域内具有可调节性，这为开发下一代光电器件和光子器件（如红外光电探测器和传感器）提供了独特的机会。这篇综述文章的核心目的是通过回顾迄今为止报道的综合文献，突出简并或重掺杂MOX纳米晶体独特而非凡的等离子体特性。特别是，分别讨论了每种MOX NC（ZnO、CdO、InO和WO）掺杂不同掺杂剂的文献。除了讨论最常用的胶体合成方法外，还详细讨论了纳米晶体中电荷载流子的超快动力学以及LSPR辅助热载流子的提取。最后，还介绍了MOX NCs在红外光电探测器和光伏（PV）自供电化学传感器中的未来潜在应用。

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