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混合相β-GaO:Zn/SnO面内异质结紫外光电探测器的波长调制与快速响应

Wavelength Modulation and Fast Response of Mixed-Phase β-GaO:Zn/SnO in-Plane Heterojunction Ultraviolet Photodetectors.

作者信息

Li Donglin, Deng Rui, Li Yongfeng, Jiang Dayong

机构信息

School of Materials Science and Engineering, Changchun University of Science and Technology, Changchun 130022, China.

Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education), College of Physics, Jilin University, Changchun 130012, China.

出版信息

ACS Appl Mater Interfaces. 2024 Aug 28;16(34):45156-45165. doi: 10.1021/acsami.4c07802. Epub 2024 Aug 16.

Abstract

Ultraviolet photodetectors based on wide bandgap mixed-phase β-GaO:Zn/SnO thin films formed through doping on the c-sapphire substrate (c-AlO) are prepared to construct in-plane heterojunctions employing a low-cost and simple preparation method. The mixed-phase thin film photodetectors have a low dark current of 0.74 nA, and the photo-to-dark current ratio ranges from 36.43 to 642.38 at 10 V. The photodetectors also have wavelength modulation, with response peaks ranging from 260 nm (4 mA/W) to 295 nm (1.63 A/W). Furthermore, the photodetectors have a fast response time with a rise time of 0.07 s/0.22 s and a decay time of 0.04 s/0.22 s at 1 V. The excellent performance of the devices is attributed to the reduction of V and the establishment of multiple electric fields in the mixed-phase films, which indicates the feasibility of implementing wavelength-modulated and fast-response β-GaO photodetectors using the sol-gel method.

摘要

基于通过在c面蓝宝石衬底(c-Al₂O₃)上掺杂形成的宽带隙混合相β-Ga₂O₃:Zn/SnO₂薄膜制备了紫外光电探测器,采用低成本且简单的制备方法构建面内异质结。混合相薄膜光电探测器的暗电流低至0.74 nA,在10 V时的光电流与暗电流之比在36.43至642.38之间。这些光电探测器还具有波长调制特性,响应峰值范围从260 nm(4 mA/W)到295 nm(1.63 A/W)。此外,光电探测器具有快速响应时间,在1 V时上升时间为0.07 s/0.22 s,衰减时间为0.04 s/0.22 s。器件的优异性能归因于混合相薄膜中V的减少和多个电场的建立,这表明使用溶胶-凝胶法实现波长调制和快速响应的β-Ga₂O₃光电探测器是可行的。

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