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手性 kagome 超导电性的残余费米弧调制。

Chiral kagome superconductivity modulations with residual Fermi arcs.

机构信息

Department of Physics, Southern University of Science and Technology, Shenzhen, China.

Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area, Shenzhen, China.

出版信息

Nature. 2024 Aug;632(8026):775-781. doi: 10.1038/s41586-024-07798-y. Epub 2024 Aug 21.

DOI:10.1038/s41586-024-07798-y
PMID:39169248
Abstract

Superconductivity involving finite-momentum pairing can lead to spatial-gap and pair-density modulations, as well as Bogoliubov Fermi states within the superconducting gap. However, the experimental realization of their intertwined relations has been challenging. Here we detect chiral kagome superconductivity modulations with residual Fermi arcs in KVSb and CsVSb using normal and Josephson scanning tunnelling microscopy down to 30 millikelvin with a resolved electronic energy difference at the microelectronvolt level. We observe a U-shaped superconducting gap with flat residual in-gap states. This gap shows chiral 2a × 2a spatial modulations with magnetic-field-tunable chirality, which align with the chiral 2a × 2a pair-density modulations observed through Josephson tunnelling. These findings demonstrate a chiral pair density wave (PDW) that breaks time-reversal symmetry. Quasiparticle interference imaging of the in-gap zero-energy states reveals segmented arcs, with high-temperature data linking them to parts of the reconstructed vanadium d-orbital states within the charge order. The detected residual Fermi arcs can be explained by the partial suppression of these d-orbital states through an interorbital 2a × 2a PDW and thus serve as candidate Bogoliubov Fermi states. In addition, we differentiate the observed PDW order from impurity-induced gap modulations. Our observations not only uncover a chiral PDW order with orbital selectivity but also show the fundamental space-momentum correspondence inherent in finite-momentum-paired superconductivity.

摘要

涉及有限动量配对的超导性可能导致空间隙和对密度调制,以及超导隙内的玻戈留波夫费米态。然而,它们相互交织关系的实验实现一直具有挑战性。在这里,我们使用正常和约瑟夫森扫描隧道显微镜在 30 毫开尔文以下的温度下,在微电子伏特级的分辨电子能量差下,在 KVSb 和 CsVSb 中检测到手性 kagome 超导调制和残留费米弧。我们观察到具有平坦残留隙内态的 U 形超导隙。该间隙显示出磁场可调手性的 2a×2a 空间调制,与通过约瑟夫森隧道观察到的手性 2a×2a 对密度调制相匹配。这些发现证明了打破时间反演对称性的手性对密度波 (PDW)。在隙内零能态的准粒子干涉成像中揭示了分段弧,高温数据将其与电荷有序中钒 d 轨道态的重建部分联系起来。通过轨道间 2a×2a PDW 部分抑制这些 d 轨道态,可以解释检测到的残留费米弧,因此它们可以作为候选玻戈留波夫费米态。此外,我们区分了观察到的 PDW 顺序与杂质诱导的间隙调制。我们的观察结果不仅揭示了具有轨道选择性的手性 PDW 顺序,而且还显示了有限动量配对超导性固有的空间-动量对应关系。

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