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夹在等离子体聚合碳氟化合物和铟镓钛氧化物之间的高度灵活且透明的无色聚酰亚胺基板，用于高性能柔性钙钛矿太阳能电池。

Highly flexible and transparent colorless polyimide substrate sandwiched between plasma polymerized fluorocarbon and InGaTiO for high performance flexible perovskite solar cells.

作者信息

Kim Su-Kyung, Cho Eun-Mi, Seok Hae-Jun, Kim Young-Yun, Choi Dong-Hyeok, Lee Sang-Jin, Jeon Nam Joong, Kim Han-Ki

机构信息

School of Advanced Materials Science and Engineering, Sungkyunkwan University, Suwon-si, Gyeonggi-do, Republic of Korea.

Chemical Materials Solution Center, Korea Research Institute of Chemical Technology, Daejeon, Republic of Korea.

出版信息

Sci Technol Adv Mater. 2024 Aug 6;25(1):2373041. doi: 10.1080/14686996.2024.2373041. eCollection 2024.

DOI:10.1080/14686996.2024.2373041
PMID:39169917
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11338216/
Abstract

We integrated transparent antireflective coatings and transparent electrodes onto flexible colorless polyimide (CPI) substrates to fabricate high-performance flexible perovskite solar cells. Multifunctional PPFC/CPI/IGTO substrates were fabricated by sputtering the optimal plasma-polymerized fluorocarbon (PPFC) antireflective coating and InGaTiO (IGTO) electrode films on both sides of the CPI substrate. By applying PPFC with a low refractive index (1.38) as an antireflective coating, the transparency of the PPFC/CPI/IGTO substrate increased by an additional 1.2%. In addition, owing to the amorphous characteristics of the PPFC and IGTO layers, the PPFC/CPI/IGTO substrate showed constant sheet resistance and transmittance change even after 10,000 cycles during the bending tests. The flexible perovskite solar cells, fabricated on the PPFC/CPI/IGTO substrate, exhibited an increase in current density of 1.48 mA/cm after the deposition of the PPFC antireflective coating. These results confirmed that the PPFC/CPI/IGTO substrate was durable against high-temperature treatment, flexible, and exhibited excellent electrical characteristics. This enhanced the efficiency and durability of the flexible perovskite solar cells. Moreover, the hydrophobic PPFC layer allowed the self-cleaning of inflexible perovskite solar cells. Given these attributes, the PPFC/CPI/IGTO structure has been recognized as a good choice for multifunctional substrates of flexible perovskite solar cells, presenting the potential for enhancing performance.

摘要

我们将透明抗反射涂层和透明电极集成到柔性无色聚酰亚胺（CPI）基板上，以制造高性能柔性钙钛矿太阳能电池。通过在CPI基板的两面溅射最佳的等离子体聚合碳氟化合物（PPFC）抗反射涂层和铟镓钛氧化物（IGTO）电极薄膜，制备了多功能PPFC/CPI/IGTO基板。通过应用低折射率（1.38）的PPFC作为抗反射涂层，PPFC/CPI/IGTO基板的透明度额外提高了1.2%。此外，由于PPFC和IGTO层的非晶特性，即使在弯曲测试的10000次循环后，PPFC/CPI/IGTO基板仍显示出恒定的薄层电阻和透光率变化。在PPFC/CPI/IGTO基板上制备的柔性钙钛矿太阳能电池，在沉积PPFC抗反射涂层后，电流密度增加了1.48 mA/cm²。这些结果证实，PPFC/CPI/IGTO基板耐高温处理、具有柔韧性且表现出优异的电学特性。这提高了柔性钙钛矿太阳能电池的效率和耐久性。此外，疏水的PPFC层使刚性钙钛矿太阳能电池能够自清洁。鉴于这些特性，PPFC/CPI/IGTO结构被认为是柔性钙钛矿太阳能电池多功能基板的理想选择，具有提高性能的潜力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/aa45b4fae500/TSTA_A_2373041_F0008_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/bcb369cdfadc/TSTA_A_2373041_UF0001_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/0009c8294561/TSTA_A_2373041_F0001_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/74c724a335dd/TSTA_A_2373041_F0002_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/33e5e46c3833/TSTA_A_2373041_F0003_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/9d39eda0a5b0/TSTA_A_2373041_F0004_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/454591a08a6d/TSTA_A_2373041_F0005_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/dbe811360701/TSTA_A_2373041_F0006_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/0ee82437beb7/TSTA_A_2373041_F0007_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/aa45b4fae500/TSTA_A_2373041_F0008_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/bcb369cdfadc/TSTA_A_2373041_UF0001_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/0009c8294561/TSTA_A_2373041_F0001_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/74c724a335dd/TSTA_A_2373041_F0002_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/33e5e46c3833/TSTA_A_2373041_F0003_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/9d39eda0a5b0/TSTA_A_2373041_F0004_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/454591a08a6d/TSTA_A_2373041_F0005_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/dbe811360701/TSTA_A_2373041_F0006_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/0ee82437beb7/TSTA_A_2373041_F0007_OC.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/051e/11338216/aa45b4fae500/TSTA_A_2373041_F0008_OC.jpg

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