Gallo Tamires, Adriano Luigi, Heymann Michael, Wrona Agnieszka, Walsh Noelle, Öhrwall Gunnar, Callefo Flavia, Skruszewicz Slawomir, Namboodiri Mahesh, Marinho Ricardo, Schulz Joachim, Valerio Joana
Lund University, Sweden.
European XFEL, Germany.
J Synchrotron Radiat. 2024 Sep 1;31(Pt 5):1285-1292. doi: 10.1107/S1600577524006611. Epub 2024 Aug 22.
One of the most challenging aspects of X-ray research is the delivery of liquid sample flows into the soft X-ray beam. Currently, cylindrical microjets are the most commonly used sample injection systems for soft X-ray liquid spectroscopy. However, they suffer from several drawbacks, such as complicated geometry due to their curved surface. In this study, we propose a novel 3D-printed nozzle design by introducing microscopic flat sheet jets that provide micrometre-thick liquid sheets with high stability, intending to make this technology more widely available to users. Our research is a collaboration between the EuXFEL and MAX IV research facilities. This collaboration aims to develop and refine a 3D-printed flat sheet nozzle design and a versatile jetting platform that is compatible with multiple endstations and measurement techniques. Our flat sheet jet platform improves the stability of the jet and increases its surface area, enabling more precise scanning and differential measurements in X-ray absorption, scattering, and imaging applications. Here, we demonstrate the performance of this new arrangement for a flat sheet jet setup with X-ray photoelectron spectroscopy, photoelectron angular distribution, and soft X-ray absorption spectroscopy experiments performed at the photoemission endstation of the FlexPES beamline at MAX IV Laboratory in Lund, Sweden.
X射线研究中最具挑战性的方面之一是将液体样品流引入软X射线束中。目前,圆柱形微射流是软X射线液体光谱学中最常用的样品注入系统。然而,它们存在一些缺点,比如由于其曲面导致几何形状复杂。在本研究中,我们通过引入微观平板射流提出了一种新颖的3D打印喷嘴设计,该射流可提供具有高稳定性的微米厚液膜,旨在使这项技术更广泛地为用户所用。我们的研究是欧洲X射线自由电子激光装置(EuXFEL)和MAX IV研究设施之间的合作。该合作旨在开发和完善一种3D打印平板喷嘴设计以及一个与多个终端站和测量技术兼容的通用喷射平台。我们的平板射流平台提高了射流的稳定性并增加了其表面积,从而能够在X射线吸收、散射和成像应用中进行更精确的扫描和差分测量。在此,我们展示了这种新的平板射流装置在瑞典隆德MAX IV实验室的FlexPES光束线的光发射终端站上进行的X射线光电子能谱、光电子角分布和软X射线吸收光谱实验中的性能。