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由CsPbBr胶体纳米晶体分散体组成的液体闪烁体中的能量沉积。

Energy deposition in liquid scintillators composed of CsPbBr colloidal nanocrystal dispersions.

作者信息

Baravaglio M, Sabot B, Maddalena F, Birowosuto M D, Dang C, Dujardin C, Mahler B

机构信息

Université Claude Bernard Lyon 1, Institut Lumière Matière UMR 5306, CNRS F-69622 Villeurbanne, France.

IRL 3288 CINTRA, CNRS-NTU-Thales, Nanyang Technological University, Research Techno Plaza, 50 Nanyang Drive, Singapore, 637553, Singapore.

出版信息

Nanoscale. 2024 Sep 19;16(36):17176-17186. doi: 10.1039/d4nr02401j.

Abstract

Liquid scintillation processes are commonly used for various applications involving radioactivity levels analysis, as well as experiments in the field of high energy physics, most commonly in the form of organic scintillating cocktails. In this paper, we explore the potential of halide perovskite nanocrystal colloidal dispersions as an alternative to those organic mixtures. After an optimization of the nanocrystals' mean size and surface chemistry, the scintillation yield of these composite mixtures is evaluated through Compton - Triple to Double Coincidence Ratio experiments and compared with commercial liquid scintillator. The obtained results shine a light on the energy deposition mechanisms in nanocrystals-based liquid scintillators.

摘要

液体闪烁过程通常用于涉及放射性水平分析的各种应用,以及高能物理领域的实验,最常见的形式是有机闪烁鸡尾酒。在本文中,我们探索了卤化物钙钛矿纳米晶体胶体分散体作为这些有机混合物替代品的潜力。在优化纳米晶体的平均尺寸和表面化学性质后,通过康普顿 - 三重与双重符合比实验评估这些复合混合物的闪烁产率,并与商业液体闪烁体进行比较。所得结果揭示了基于纳米晶体的液体闪烁体中的能量沉积机制。

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