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通过中子散射探测受限在多孔材料中的流体行为：在二氧化碳封存及强化油气开采中的应用

Probing the Behaviour of Fluids Confined in Porous Materials by Neutron Scattering: Applications to CO Sequestration and Enhanced Oil and Gas Recovery.

作者信息

Stefanopoulos Konstantinos L

机构信息

Institute of Nanoscience and Nanotechnology, National Centre for Scientific Research "Demokritos", 153 10 Ag. Paraskevi, Athens, Greece.

出版信息

Chempluschem. 2024 Dec;89(12):e202400353. doi: 10.1002/cplu.202400353. Epub 2024 Oct 24.

DOI:10.1002/cplu.202400353
PMID:39206570
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11639646/
Abstract

The current review presents a discussion on the utility of neutron scattering, with emphasis on neutron total scattering and small-angle neutron scattering (SANS), to explore the structural properties and the phase behaviour of fluids confined in nanopores. The effectiveness of contrast matching SANS on the evaluation of accessibility of porous materials to invading fluids is highlighted too. This review provides also an overview regarding the neutron scattering studies on the structure and the accessibility of greenhouse gases in the complex pore network of geomaterials, with applications to CO geological sequestration and enhanced oil and gas recovery.

摘要

本综述讨论了中子散射的应用，重点是中子全散射和小角中子散射（SANS），以探索限制在纳米孔中的流体的结构性质和相行为。还强调了对比匹配SANS在评估多孔材料对侵入流体的可及性方面的有效性。本综述还概述了关于地质材料复杂孔隙网络中温室气体的结构和可及性的中子散射研究，并应用于二氧化碳地质封存以及提高油气采收率。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/d4a1a065e516/CPLU-89-e202400353-g008.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/76a85a77b33d/CPLU-89-e202400353-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/e5b9cef3cbde/CPLU-89-e202400353-g004.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/86e3821f5703/CPLU-89-e202400353-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/03f519ec2228/CPLU-89-e202400353-g011.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/3904f70a1ec2/CPLU-89-e202400353-g013.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/3bb625915a8f/CPLU-89-e202400353-g010.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/76a85a77b33d/CPLU-89-e202400353-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/e5b9cef3cbde/CPLU-89-e202400353-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/84b1dab9e71a/CPLU-89-e202400353-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/183c/11639646/645135a4fcab/CPLU-89-e202400353-g014.jpg
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本文引用的文献

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In Situ Neutron Diffraction of Zn-MOF-74 Reveals Nanoconfinement-Induced Effects on Adsorbed Propene.锌基金属有机框架材料-74（Zn-MOF-74）的原位中子衍射揭示了纳米限域对吸附丙烯的影响。
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Neutron Scattering Studies of Heterogeneous Catalysis.
中子散射在多相催化研究中的应用。
Chem Rev. 2023 Jul 12;123(13):8638-8700. doi: 10.1021/acs.chemrev.3c00101. Epub 2023 Jun 14.
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Influence Factors and Feasibility Evaluation on Geological Sequestration of CO in Coal Seams: A Review.煤层中CO地质封存的影响因素与可行性评价综述
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