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低凝点柴油的使用加剧了中国寒冷地区的冬季雾霾。

Low-condensation diesel use contributes to winter haze in cold regions of China.

作者信息

Song Weiwei, Wang Mengying, Zhao Yixuan, Bo Yu, Yao Wanying, Chen Ruihan, Wang Xianshi, Wang Xiaoyan, Li Chunhui, He Kebin

机构信息

State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin, 150090, China.

State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China.

出版信息

Environ Sci Ecotechnol. 2024 Jul 17;22:100456. doi: 10.1016/j.ese.2024.100456. eCollection 2024 Nov.

Abstract

The application of low-condensation diesel in cold regions with extremely low ambient temperatures (-14 to -29 °C) has enabled the operation of diesel vehicles. Still, it may contribute to heavy haze pollution in cold regions during winter. Here we examine pollutant emissions from low-condensation diesel in China. We measure the emissions of elemental carbon (EC), organic carbon (OC), and elements, including heavy metals such as arsenic (As). Our results show that low-condensation diesel increased EC and OC emissions by 2.5 and 2.6 times compared to normal diesel fuel, respectively. Indicators of vehicular sources, including EC, As, lead (Pb), cadmium (Cd), chromium (Cr), nickel (Ni), and manganese (Mn), increased by approximately 20.2-162.5% when using low-condensation diesel. Seasonal variation of vehicular source indicators, observed at road site ambient environments revealed the enhancement of PM pollution by the application of low-condensation diesel in winter. These findings suggest that -35# diesel, a low-cetane index diesel, may enhance air pollution in winter, according to a dynamometer test conducted in laboratory. It raises questions about whether higher emissions are released if -35# diesel is applied to running vehicles in real-world cold ambient environments.

摘要

低凝柴油在环境温度极低(-14至-29°C)的寒冷地区的应用,使得柴油车辆能够运行。然而,这可能会导致冬季寒冷地区出现严重的雾霾污染。在此,我们研究了中国低凝柴油的污染物排放情况。我们测量了元素碳(EC)、有机碳(OC)以及包括砷(As)等重金属在内的元素的排放。我们的结果表明,与普通柴油相比,低凝柴油使EC和OC排放分别增加了2.5倍和2.6倍。使用低凝柴油时,包括EC、As、铅(Pb)、镉(Cd)、铬(Cr)、镍(Ni)和锰(Mn)在内的车辆源指标增加了约20.2 - 162.5%。在道路现场环境中观察到的车辆源指标的季节性变化表明,冬季使用低凝柴油会加剧颗粒物污染。根据在实验室进行的台架试验,这些发现表明,十六烷值指数较低的-35#柴油可能会加剧冬季空气污染。这引发了一个问题,即在实际寒冷的环境中,如果将-35#柴油应用于行驶中的车辆,是否会释放更高的排放量。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d714/11364129/8399b0a81885/ga1.jpg

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