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低温下增强的柴油排放:细颗粒物中的有害物质。

Enhanced diesel emissions at low ambient temperature: hazardous materials in fine particles.

机构信息

State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China.

State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, 100871 Beijing, China.

出版信息

J Hazard Mater. 2023 May 5;449:131011. doi: 10.1016/j.jhazmat.2023.131011. Epub 2023 Feb 15.

Abstract

The emission of fine particles (PM) from diesel trucks is enhanced by low ambient temperatures, which is a fact that has attracted considerable attention. Carbonaceous matter and polycyclic aromatic hydrocarbons (PAHs) are the dominant hazardous materials in PM. These materials induce severe adverse effects on air quality and human health and contribute to climate change. The emissions from heavy- and light-duty diesel trucks were tested at an ambient temperature of - 20 to - 13 ℃ and 18-24 ℃. This is the first study to quantify the enhanced carbonaceous matter and PAH emissions from diesel trucks at very low ambient temperatures based on an on-road emission test system. Features affecting diesel emissions, including driving speed, vehicle type, and engine certification level, were considered. The emissions of organic carbon, elemental carbon, and PAHs significantly increased from - 20 to - 13 ℃. The empirical results revealed that intensive abatement of diesel emissions at low ambient temperatures could benefit human health and have a positive influence on climate change. Considering the widespread applications worldwide, an investigation into diesel emissions of carbonaceous matter and PAHs in fine particles at low ambient temperatures is urgently required.

摘要

柴油卡车在环境温度较低时会增加细颗粒物(PM)的排放,这是一个引起广泛关注的事实。碳质物质和多环芳烃(PAHs)是 PM 中主要的有害物质。这些物质对空气质量和人类健康造成严重影响,并导致气候变化。在环境温度为-20 至-13°C 和 18-24°C 的情况下,对重型和轻型柴油卡车的排放进行了测试。这是首次基于道路排放测试系统,在极低环境温度下定量评估柴油卡车碳质物质和 PAH 排放增强的研究。考虑了影响柴油排放的特征,包括行驶速度、车辆类型和发动机认证级别。有机碳、元素碳和 PAHs 的排放量从-20°C 到-13°C 显著增加。实证结果表明,在环境温度较低时,加强对柴油排放的控制将有益于人类健康,并对气候变化产生积极影响。考虑到全球范围内的广泛应用,迫切需要对低温下细颗粒物中碳质物质和 PAHs 的柴油排放进行调查。

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