Arunachalam Sankara, Lin Marcus, Daniel Dan
Droplet Lab, Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Saudi Arabia.
Soft Matter. 2024 Oct 2;20(38):7583-7591. doi: 10.1039/d4sm00601a.
Previously, we and others have used cantilever-based techniques to measure droplet friction on various surfaces, but typically at low speeds < 1 mm s; at higher speeds, friction measurements become inaccurate because of ringing artefacts. Here, we are able to eliminate the ringing noise using a critically damped cantilever. We measured droplet friction on a superhydrophobic surface over a wide range of speeds = 10-10 m s and identified two regimes corresponding to two different physical origins of droplet friction. At low speeds < 1 cm s, the droplet is in contact with the top-most solid (Cassie-Baxter), and friction is dominated by contact-line pinning with force that is independent of . In contrast, at high speeds > 1 cm s, the droplet lifts off the surface, and friction is dominated by viscous dissipation in the air layer with ∝ consistent with Landau-Levich-Derjaguin predictions. The same scaling applies for superhydrophobic and underwater superoleophobic surfaces despite their very different surface topographies and chemistries, , the friction scaling law derived here is universal.
此前,我们和其他研究人员已使用基于悬臂梁的技术来测量不同表面上液滴的摩擦力,但通常是在低速(<1毫米/秒)下进行;在较高速度下,由于振铃伪像,摩擦力测量变得不准确。在这里,我们能够使用临界阻尼悬臂梁消除振铃噪声。我们在超疏水表面上测量了广泛速度范围(10^-10米/秒)内的液滴摩擦力,并确定了与液滴摩擦力的两种不同物理起源相对应的两种状态。在低速(<1厘米/秒)下,液滴与最上层固体接触(卡西 - 巴克斯特状态),摩擦力主要由接触线钉扎主导,其力与速度无关。相比之下,在高速(>1厘米/秒)下,液滴离开表面,摩擦力主要由空气层中的粘性耗散主导,其中与速度成正比,这与朗道 - 列维奇 - 杰里亚金的预测一致。尽管超疏水和水下超疏油表面的表面形貌和化学性质截然不同,但相同的标度关系仍然适用,即这里推导的摩擦标度定律是通用的。