Rudno-Rudziński Wojciech, Gawełczyk Michał, Podemski Paweł, Cybula Ewelina, Gorantla Sandeep, Balasubramanian Ramasubramanian, Sichkovskyi Vitalii, Willinger Amnon J, Eisenstein Gadi, Reithmaier Johann P, Sęk Grzegorz
Department of Experimental Physics, Wrocław University of Science and Technology, St. Wyspiańskiego 27, 50-370 Wrocław, Poland.
Institute of Theoretical Physics, Wrocław University of Science and Technology, St. Wyspiańskiego 27, 50-370 Wrocław, Poland.
ACS Appl Mater Interfaces. 2024 Sep 25;16(38):51150-51162. doi: 10.1021/acsami.4c12061. Epub 2024 Sep 13.
Integrating light emitters based on III-V materials with silicon-based electronics is crucial for further increase in data transfer rates in communication systems since the indirect bandgap of silicon prevents its direct use as a light source. We investigate here InAs/InGaAlAs quantum dot (QD) structures grown directly on 5° off-cut Si substrate and emitting light at 1.5 μm, compatible with established telecom platform. Using different dislocation defect filtering layers, exploiting strained superlattices, and supplementary QD layers, we mitigate the effects of lattice constant and thermal expansion mismatches between III-V materials and Si during growth. Complementary optical spectroscopy techniques, i.e. photoreflectance and temperature-, time- and polarization-resolved photoluminescence, allow us to determine the optical quality and application potential of the obtained structures by comparing them to a reference sample-state-of-the-art QDs grown on InP. Experimental findings are supported by calculations of excitonic states and optical transitions by combining multiband • and configuration-interaction methods. We show that our design of structures prevents the generation of a considerable density of defects, as intended. The emission of Si-based structures appears to be much broader than for the reference dots, due to the creation of different QD populations which might be a disadvantage in particular laser applications, however, could be favorable for others, e.g., in broadly tunable devices, sensors, or optical amplifiers. Eventually, we identify the overall most promising combination of defect filtering layers and discuss its advantages and limitations and prospects for further improvements.
将基于III-V族材料的发光器与硅基电子器件集成,对于进一步提高通信系统中的数据传输速率至关重要,因为硅的间接带隙使其无法直接用作光源。我们在此研究直接生长在5°斜切硅衬底上、发射1.5μm光的InAs/InGaAlAs量子点(QD)结构,该结构与已建立的电信平台兼容。通过使用不同的位错缺陷过滤层、利用应变超晶格和补充量子点层,我们减轻了III-V族材料与硅在生长过程中晶格常数和热膨胀失配的影响。互补的光谱技术,即光反射光谱以及温度、时间和偏振分辨光致发光光谱,使我们能够通过将所得结构与在InP上生长的参考样品——最先进的量子点进行比较,来确定其光学质量和应用潜力。通过结合多带和组态相互作用方法对激子态和光学跃迁进行计算,支持了实验结果。我们表明,我们的结构设计按预期防止了大量缺陷的产生。由于形成了不同的量子点群体,硅基结构的发射似乎比参考量子点宽得多,这在特定的激光应用中可能是一个缺点,然而,在其他应用中,例如在宽可调谐器件、传感器或光放大器中可能是有利的。最终,我们确定了缺陷过滤层的总体最有前景的组合,并讨论了其优点、局限性以及进一步改进的前景。