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Half-life determination of Ga.

作者信息

Dong Jiangpeng, Bai Tao, Dai Yihua, Fan Jinlong, Zhao Keqi, Song Xiaojing, Shi Quanlin, Li Zhiming

机构信息

Northwest Institute of Nuclear Technology, Xi'an, 710024, China.

Northwest Institute of Nuclear Technology, Xi'an, 710024, China.

出版信息

Appl Radiat Isot. 2024 Dec;214:111517. doi: 10.1016/j.apradiso.2024.111517. Epub 2024 Sep 10.

Abstract

Gallium-72 is an important Comprehensive Nuclear-Test-Ban Treaty relevant radionuclide that arouses significant interest. However, the reported half-lives of Ga are discrepant. In the current work, three solution samples of different concentrations were prepared and sequentially measured by a high-purity Germanium (HPGe) spectrometer. The count rates as a function of time of the 834.1 keV and 630.0 keV γ-lines were followed for the half-life determination. Through mass normalization, the datasets of three samples are combined and the statistical uncertainties are reduced. Half-life values were derived from datasets of each sample and mass normalization and corresponding complete uncertainty budgets are presented. The final half-life determined for Ga is 13.94 (2) h, showing a deviation of 1.12% from the last nuclear data sheets (NDS) recommended value. Comparing with the values of previous publications, the result from this work is smaller than most results and consistent with the latest value which has one large uncertainty. A recommended value of 14.07 (3) h is estimated using the power-moderated mean (PMM) method.

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