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基于生物质的纳米纤维膜复合材料与木聚糖衍生的碳点用于食品实际样品中亚硝酸盐的荧光检测

Biomass based nanofiber membrane composite with xylan derived carbon dots for fluorescence detection nitrite in food real samples.

作者信息

Chen Zhiyuan, Zhang Yingying, Feng Xiuyuan, Cui Xiaoci, Xiao Huining, Yang Anquan, Xie Min, Xiong Ranhua, Cheng Weixia, Huang Chaobo

机构信息

Joint Laboratory of Advanced Biomedical Materials (NFU-UGent), Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Chemical Engineering, Nanjing Forestry University (NFU), Nanjing 210037, China.

Joint Laboratory of Advanced Biomedical Materials (NFU-UGent), Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Chemical Engineering, Nanjing Forestry University (NFU), Nanjing 210037, China.

出版信息

Int J Biol Macromol. 2024 Sep 14;280(Pt 1):135693. doi: 10.1016/j.ijbiomac.2024.135693.

Abstract

In our latest research endeavor, we are proud to present an innovative approach to the synthesis of carbon dots (CDs) derived from the biomass xylan, which we have termed P-CDs. These P-CDs are meticulously integrated with a state-of-the-art biomass nanofiber membrane composed of polycaprolactone (PCL) and polylactic acid (PLA), resulting in the creation of a novel solid-state fluorescent sensor, designated as NFP-CDs. This cutting-edge sensor has been meticulously engineered for the highly sensitive and specific detection of nitrite ions (NO), a critical parameter in various fields. The NFP-CDs sensor stands out for its user-friendly design, cost-effective production, and portable nature, making it an ideal choice for rapid and visible nitrite ion detection. It exhibits an extraordinary response time of less than 1 s, which is a testament to its high sensitivity. Furthermore, the sensor demonstrates exceptional selectivity and specificity, with a remarkably low detection threshold of 0.36 μM. This is achieved through a sophisticated dual detection mechanism that synergistically combines colorimetric and spectral analyses, ensuring accurate and reliable results. In addition to its impressive technical specifications, the NFP-CDs sensor has been rigorously tested and validated for its efficacy in detecting nitrite ions in real-world samples. These samples include a diverse range of food products such as rock sugar, preserved mustard, kimchi, and canned fish. The sensor has demonstrated a remarkable recovery rate, which varies from 99 % to 106 %, highlighting its potential for practical application in nitrite ion detection. This research not only offers a robust and effective strategy for the detection of nitrite ions but also carries profound implications for enhancing food safety and bolstering environmental monitoring efforts. The development of the NFP-CDs sensor represents a significant step forward in the field of sensor technology, providing a powerful tool for the detection of nitrite ions and contributing to the broader goals of public health and environmental stewardship.

摘要

在我们最新的研究工作中,我们自豪地展示了一种创新方法,用于合成源自生物质木聚糖的碳点(CDs),我们将其命名为P-CDs。这些P-CDs与由聚己内酯(PCL)和聚乳酸(PLA)组成的先进生物质纳米纤维膜精心整合,从而创造出一种新型固态荧光传感器,命名为NFP-CDs。这种前沿传感器经过精心设计,用于高灵敏度和特异性地检测亚硝酸根离子(NO),这是各个领域的一个关键参数。NFP-CDs传感器以其用户友好的设计、经济高效的生产和便携性脱颖而出,使其成为快速且可视化亚硝酸根离子检测的理想选择。它具有不到1秒的非凡响应时间,这证明了其高灵敏度。此外,该传感器表现出卓越的选择性和特异性,检测阈值低至0.36 μM。这是通过一种复杂的双检测机制实现的,该机制将比色分析和光谱分析协同结合,确保结果准确可靠。除了令人印象深刻的技术规格外,NFP-CDs传感器还经过了严格测试和验证,以证明其在检测实际样品中亚硝酸根离子方面的功效。这些样品包括各种食品,如冰糖、榨菜、泡菜和罐头鱼。该传感器显示出显著的回收率,从99%到106%不等,突出了其在亚硝酸根离子检测中的实际应用潜力。这项研究不仅为亚硝酸根离子的检测提供了一种强大而有效的策略,而且对加强食品安全和促进环境监测工作具有深远意义。NFP-CDs传感器的开发代表了传感器技术领域向前迈出的重要一步,为亚硝酸根离子的检测提供了一个强大工具,并有助于实现公共卫生和环境管理的更广泛目标。

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