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通过电流诱导退火实现的硒化铋纳米带之间的超低接触热阻

Ultralow Contact Thermal Resistance between Bismuth Selenide Nanoribbons Achieved by Current-Induced Annealing.

作者信息

Xiong Yucheng, Li Shouhang, Wang Renzong, Cheng Zhe, Yang Juekuan, Li Deyu, Liu Xiangjun, Xu Dongyan

机构信息

Institute of Micro/Nano Electromechanical System, College of Mechanical Engineering, Donghua University, Shanghai 201620, China.

Department of Mechanical and Automation Engineering, The Chinese University of Hong Kong, Shatin, New Territories, Hong Kong Special Administrative Region, China.

出版信息

ACS Appl Mater Interfaces. 2024 Oct 23;16(42):57824-57831. doi: 10.1021/acsami.4c10789. Epub 2024 Oct 10.

Abstract

Thermal resistance at interfaces/contacts stands as a persistent and increasingly critical issue, which hinders ultimate scaling and the performance of electronic devices. Compared to the extensive research on contact electrical resistance, contact thermal resistance and its mitigation strategies have received relatively less attention. Here, we report on an effective, in situ, and energy-efficient approach for enhancing thermal transport through the contact between semiconducting nanoribbons. By applying microampere-level electrical currents to the contact between BiSe nanoribbons, we demonstrate that the contact thermal resistance between two nanoribbon segments is reduced dramatically by a factor of 4, rendering the total thermal resistance of two ribbon segments with a contact approximately the same as that of the corresponding single continuous nanoribbon of the same length. Analysis suggests that the ultralow contact thermal resistance is due to enhanced phonon transmission as a result of enhanced adhesion energy at the contact, with marginal contributions from direct electron-phonon coupling, even for ohmic contacts. Our work introduces a broadly applicable electrical treatment approach to various contacts between conducting and semiconducting materials, which has important implications for the design and operation of nanoelectronic devices and energy converters.

摘要

界面/接触处的热阻一直是个持续且日益关键的问题,它阻碍了电子器件的最终缩放和性能提升。与对接触电阻的广泛研究相比,接触热阻及其缓解策略受到的关注相对较少。在此,我们报道了一种有效、原位且节能的方法,用于增强通过半导体纳米带之间接触的热传输。通过向BiSe纳米带之间的接触施加微安级电流,我们证明两个纳米带段之间的接触热阻大幅降低了4倍,使得有接触的两个带段的总热阻与相同长度的相应单个连续纳米带的热阻大致相同。分析表明,超低接触热阻是由于接触处粘附能增强导致声子传输增强,即使对于欧姆接触,直接电子 - 声子耦合的贡献也很小。我们的工作为导电和半导体材料之间的各种接触引入了一种广泛适用的电处理方法,这对纳米电子器件和能量转换器的设计与运行具有重要意义。

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