Godini Hamid Reza, Bhasin Madan Mohan
Chair of Process Dynamics and Operation, Technische Universität Berlin, Strasse des 17. Juni 135, 10623 Berlin, Germany.
Innovative Catalytic Solutions, LLC, 2048 Smith Road, Charleston, WV 25324, USA.
Molecules. 2024 Sep 30;29(19):4649. doi: 10.3390/molecules29194649.
Extensive data on the characteristics and performance of the catalysts synthesized and tested for methane oxidative coupling (OCM) is available in thousands of reports published during the last four decades. Revisiting and analyzing the general trends recognizable in those data could improve the current understanding of the catalyst functionality under different reaction conditions. This is instrumental in determining the direction of future research aiming for more efficient OCM catalysts and reactors. These are the subjects of the comprehensive analysis reported in this paper, which covers the main aspects associated with the analysis of the OCM catalytic performance, including the catalyst characteristics, reaction mechanism, and reactor operation. Special attention was devoted to analyzing these aspects in the framework of thermal-reaction engineering and, accordingly, critically reviewing the reported catalytic performances in the literature.
在过去四十年间发表的数千份报告中，有关于为甲烷氧化偶联（OCM）合成和测试的催化剂的特性及性能的大量数据。回顾和分析这些数据中可识别的总体趋势，有助于增进当前对不同反应条件下催化剂功能的理解。这对于确定旨在研发更高效OCM催化剂和反应器的未来研究方向至关重要。这些就是本文所报道的综合分析的主题，该分析涵盖了与OCM催化性能分析相关的主要方面，包括催化剂特性、反应机理和反应器操作。特别关注在热反应工程框架内对这些方面进行分析，并据此严格审视文献中报道的催化性能。
