Chen Siao, Zheng Xuchen, Gao Yang, Ping Xinyu, Xue Yurui, Li Yuliang
CAS Key Laboratory of Organic Solids, Institute of Chemistry Chinese Academy of Sciences, Beijing 100190, China.
School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China.
Precis Chem. 2024 Apr 9;2(7):355-375. doi: 10.1021/prechem.3c00125. eCollection 2024 Jul 22.
Graphdiyne (GDY) science is a new and rapidly developing interdisciplinary field that touches on various areas of chemistry, physics, information science, material science, life science, environmental science, and so on. The rapid development of GDY science is part of the trend in development of carbon materials. GDY, with its unique structure and fascinating properties, has greatly promoted fundamental research toward practical applications of carbon materials. Many important applications, such as catalysis and energy conversion, have been reported. In particular, GDY has shown great potential for application in the field of catalysis. Scientists have precisely synthesized a series of GDY-based multiscale catalysts and applied them in various energy conversion and catalysis research, including ammonia synthesis, hydrogen production, CO conversion, and chemical-to-electrical energy conversion. In this paper, we systematically review the advances in the precisely controlled synthesis of GDY and aggregated structures, and the latest progress with GDY in catalysis and energy conversion.
石墨炔（GDY）科学是一个新兴且发展迅速的跨学科领域，涉及化学、物理、信息科学、材料科学、生命科学、环境科学等各个领域。GDY科学的快速发展是碳材料发展趋势的一部分。GDY凭借其独特的结构和迷人的性质，极大地推动了碳材料从基础研究到实际应用的进程。已经报道了许多重要应用，如催化和能量转换。特别是，GDY在催化领域显示出了巨大的应用潜力。科学家们精确合成了一系列基于GDY的多尺度催化剂，并将其应用于各种能量转换和催化研究中，包括氨合成、制氢、CO转化以及化学能到电能的转换。在本文中，我们系统地综述了GDY及其聚集结构精确控制合成方面的进展，以及GDY在催化和能量转换方面的最新进展。
