Sun Jiali, Dang Yuying, Sun Xiaoyan, Heumann Saskia, Ding Yuxiao
Institution: Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Middle Road 18, Tianshui, Lanzhou, 730000, China.
Max Planck Institute for Chemical Energy Conversion, Stiftstrasse 34-36, 45470, Mülheim an der Ruhr, Germany.
ChemSusChem. 2025 Feb 1;18(3):e202401340. doi: 10.1002/cssc.202401340. Epub 2024 Oct 30.
Carbon materials, whose structural and electronic properties can be fine-tuned, are promising material solutions for many energy-related systems. However, due to the lack of fundamental understanding of the carbon surface chemistry, especially when they are used in electrolytes, the rapid development of carbon as electrodes has led to many widely accepted misunderstandings. Focusing on the case of carbon-based electrode for water splitting, this Viewpoint tries to highlight the main problems of the area and demonstrates/presents the dynamic carbon surface chemistry in the application. The role of carbon as an anode for water splitting is revealed and if it can be practically used in water splitting is discussed.
碳材料的结构和电子特性可进行微调,是许多与能源相关系统颇具前景的材料解决方案。然而,由于对碳表面化学缺乏基本认识,尤其是当它们用于电解质时,碳作为电极的快速发展导致了许多被广泛接受的误解。以用于水分解的碳基电极为例,本观点试图突出该领域的主要问题,并展示应用中动态的碳表面化学。揭示了碳作为水分解阳极的作用,并讨论了其是否能实际用于水分解。