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室温下的光谱可调谐超快长波红外探测

Spectrally Tunable Ultrafast Long Wave Infrared Detection at Room Temperature.

作者信息

Guo Tianyi, Chandra Sayan, Dasgupta Arindam, Shabbir Muhammad Waqas, Biswas Aritra, Chanda Debashis

机构信息

Department of Physics, University of Central Florida, Orlando, Florida 32816, United States.

NanoScience Technology Center, University of Central Florida, Orlando, Florida 32826, United States.

出版信息

Nano Lett. 2024 Nov 20;24(46):14678-14685. doi: 10.1021/acs.nanolett.4c03832. Epub 2024 Nov 6.

Abstract

Room-temperature longwave infrared (LWIR) detectors are preferred over cryogenically cooled solutions due to the cost effectiveness and ease of operation. The performance of present uncooled LWIR detectors such as microbolometers, is limited by reduced sensitivity, slow response time, and the lack of dynamic spectral tunability. Here, we present a graphene-based efficient room-temperature LWIR detector with high detectivity and fast response time utilizing its tunable optical and electronic characteristics. The inherent weak light absorption is enhanced by Dirac plasmons on the patterned graphene coupled to an optical cavity. The absorbed energy is converted into photovoltage by the Seebeck effect with an asymmetric carrier generation environment. Further, dynamic spectral tunability in the 8-12 μm LWIR band is achieved by electrostatic gating. The proposed detection platform paves the path to a fresh generation of uncooled graphene-based LWIR photodetectors for wide ranging applications such as molecular sensing, medical diagnostics, military, security and space.

摘要

由于成本效益高且操作简便,室温长波红外(LWIR)探测器比低温冷却解决方案更受青睐。目前诸如微测辐射热计等非制冷LWIR探测器的性能受到灵敏度降低、响应时间缓慢以及缺乏动态光谱可调性的限制。在此,我们展示了一种基于石墨烯的高效室温LWIR探测器,它利用其可调谐的光学和电子特性,具有高探测率和快速响应时间。通过与光学腔耦合的图案化石墨烯上的狄拉克等离子体增强了固有的弱光吸收。在不对称载流子产生环境下,吸收的能量通过塞贝克效应转化为光电压。此外,通过静电门控实现了8 - 12μm LWIR波段的动态光谱可调性。所提出的检测平台为新一代基于石墨烯的非制冷LWIR光电探测器铺平了道路,可用于分子传感、医学诊断、军事、安全和太空等广泛应用。

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