Golenić Neven, de Gironcoli Stefano, Despoja Vito
Department of Physics, University of Zagreb, Bijenička 32, 10000, Zagreb, Croatia.
Scuola Internazionale Superiore di Studi Avanzati (SISSA), Via Bonomea 265, 34136 Trieste, Italy.
Nanophotonics. 2024 Apr 15;13(15):2765-2780. doi: 10.1515/nanoph-2023-0841. eCollection 2024 Jul.
Converting transverse photons into longitudinal two-dimensional plasmon--polaritons (2D-PP) and vice versa presents a significant challenge within the fields of photonics and plasmonics. Therefore, understanding the mechanism which increases the photon - 2D-PP conversion efficiency could significantly contribute to those efforts. In this study, we theoretically examine how efficiently incident radiation, when scattered by a silver spherical nanoparticle (Ag-NP), can be transformed into 2D-PP within van der Waals (vdW) heterostructures composed of hexagonal boron nitride and graphene (hBN/Gr composites). We show that the Dirac plasmon (DP) excitation efficiency depends on the Ag-NP radius as , and decreases exponentially with Ag-NP height , so that for a certain Ag-NP geometry up to 25 % of the incident electrical field is channeled into the DP. We demonstrate that the linear plasmons (LPs) excitation efficiency can be manipulated by changing the graphene-graphene distance Δ (or hBN thickness) or by changing the number of graphene layers . By increasing Δ and/or the LPs move towards smaller wave vectors and become accessible by the Ag-NP dipole field, so that for ≥ 5 the excitation of more than one LP is possible. These results are supported by recent scattering-type scanning near-field optical microscopy (s-SNOM) measurements. Furthermore, we show that Ag-NPs with specific parameters preferentially hybridizes with DPs of a particular wavelength , facilitating selective excitation of DPs. The obtained tuning possibilities could have a significant impact on applied plasmonics, photonics or optoelectronics.
将横向光子转换为纵向二维表面等离激元-极化激元(2D-PP),反之亦然,这在光子学和等离子体学领域是一项重大挑战。因此,了解提高光子与2D-PP转换效率的机制,可能会对这些研究工作做出重大贡献。在本研究中,我们从理论上研究了入射辐射在被银球形纳米颗粒(Ag-NP)散射时,如何在由六方氮化硼和石墨烯组成的范德华(vdW)异质结构(hBN/Gr复合材料)中高效地转换为2D-PP。我们表明,狄拉克表面等离激元(DP)的激发效率取决于Ag-NP半径 ,并随Ag-NP高度 呈指数下降,因此对于特定的Ag-NP几何结构,高达25%的入射电场会被引导到DP中。我们证明,线性表面等离激元(LP)的激发效率可以通过改变石墨烯-石墨烯间距Δ(或hBN厚度)或改变石墨烯层数 来控制。通过增加Δ和/或 ,LP向更小的波矢 移动,并可被Ag-NP偶极场激发,因此对于 ≥ 5,可以激发多个LP。这些结果得到了最近散射型扫描近场光学显微镜(s-SNOM)测量的支持。此外,我们表明具有特定参数的Ag-NP优先与特定波长 的DP杂交,有利于DP的选择性激发。所获得的调谐可能性可能会对应用等离子体学、光子学或光电子学产生重大影响。