Lin Yu-Tsung, Hassanfiroozi Amir, Jiang Wei-Rou, Liao Mei-Yi, Lee Wen-Jen, Wu Pin Chieh
Department of Photonics, National Cheng Kung University, Tainan 70101, Taiwan, ROC.
Department of Applied Chemistry, National Pingtung University, Pingtung 90003, Taiwan, ROC.
Nanophotonics. 2021 Dec 22;11(11):2701-2709. doi: 10.1515/nanoph-2021-0640. eCollection 2022 Jun.
Mie resonances have recently attracted much attention in research on dielectric metasurfaces, owning to their enriched multipole resonances, negligible optical loss, and efficient light emitter integration. Although there is a rapid advancement in this field, some fundamental developments are still required to provide a simpler and more versatile paradigm for photoluminescence (PL) control. In this work, we proposed that an all-dielectric coherent metasurface can engineer the PL response by tuning the array size. Such PL manipulation is attributed to the collective Mie resonances that mediate the inter-unit interactions between unit elements and alter the PL intensity. Metasurfaces with different chip sizes are utilized to explore the array size effect on the collective Mie resonances, field enhancement, and Q-factor in TiO metasurfaces. Incorporating the all-dielectric coherent metasurface with fluorescent photon emitters, we performed the dependence of PL enhancement on array size, which achieves an enhancement factor of ∼10 at the central area of a 90 × 90 μm TiO metasurface array. These findings provide an additional degree of freedom to engineer the near-field confinement and enhancement, allowing one to manipulate incoherent photon emission and tune light-matter interaction at the nanoscale.
米氏共振最近在介电超表面研究中备受关注,这归因于其丰富的多极共振、可忽略不计的光学损耗以及高效的发光体集成。尽管该领域发展迅速,但仍需要一些基础进展来提供一种更简单、更通用的光致发光(PL)控制模式。在这项工作中,我们提出全介质相干超表面可以通过调整阵列尺寸来调控PL响应。这种PL操控归因于集体米氏共振,它介导了单元元件之间的单元间相互作用并改变了PL强度。利用具有不同芯片尺寸的超表面来探究阵列尺寸对TiO超表面中集体米氏共振、场增强和品质因数的影响。将全介质相干超表面与荧光光子发射体相结合,我们研究了PL增强对阵列尺寸的依赖性,在90×90μm TiO超表面阵列的中心区域实现了约10的增强因子。这些发现为设计近场限制和增强提供了额外的自由度,使人们能够在纳米尺度上操控非相干光子发射并调整光与物质的相互作用。