Takagi Rina, Hirakida Ryosuke, Settai Yuki, Oiwa Rikuto, Takagi Hirotaka, Kitaori Aki, Yamauchi Kensei, Inoue Hiroki, Yamaura Jun-Ichi, Nishio-Hamane Daisuke, Itoh Shinichi, Aji Seno, Saito Hiraku, Nakajima Taro, Nomoto Takuya, Arita Ryotaro, Seki Shinichiro
Department of Applied Physics, University of Tokyo, Tokyo, Japan.
Institute of Engineering Innovation, University of Tokyo, Tokyo, Japan.
Nat Mater. 2025 Jan;24(1):63-68. doi: 10.1038/s41563-024-02058-w. Epub 2024 Dec 13.
Magnetic information is usually stored in ferromagnets, where the ↑ and ↓ spin states are distinguishable due to time-reversal symmetry breaking. These states induce opposite signs of the Hall effect proportional to magnetization, which is widely used for their electrical read-out. By contrast, conventional antiferromagnets with a collinear antiparallel spin configuration cannot host such functions, because of symmetry (time-reversal followed by translation t symmetry) and lack of macroscopic magnetization. Here we report the experimental observation of a spontaneous Hall effect in the collinear antiferromagnet FeS at room temperature. In this compound, the ↑↓ and ↓↑ spin states induce opposite signs of the spontaneous Hall effect. Our analysis suggests that this does not reflect magnetization, but rather originates from a fictitious magnetic field associated with the -symmetry-broken antiferromagnetic order. The present results pave the way for electrical reading and writing of the ↑↓ and ↓↑ spin states in conductive systems at room temperature, and suggest that -symmetry-broken collinear antiferromagnets can serve as an information medium with vanishingly small magnetization.
磁信息通常存储在铁磁体中,由于时间反演对称性破缺,其中↑和↓自旋态是可区分的。这些状态会诱导出与磁化强度成正比的相反符号的霍尔效应,这在其电读出中得到了广泛应用。相比之下,具有共线反平行自旋构型的传统反铁磁体无法具备此类功能,因为其具有对称性(时间反演和平移t对称性)且缺乏宏观磁化强度。在此,我们报告了在室温下共线反铁磁体FeS中自发霍尔效应的实验观测结果。在这种化合物中,↑↓和↓↑自旋态会诱导出自发霍尔效应的相反符号。我们的分析表明,这并非反映磁化强度,而是源于与对称性破缺的反铁磁序相关的虚拟磁场。目前的结果为室温下导电系统中↑↓和↓↑自旋态的电读写铺平了道路,并表明对称性破缺的共线反铁磁体可作为磁化强度极小的信息介质。