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表面等离子体共振增强极性/半极性InGaN/GaN发射的空间和时间分辨特性

Spatial and time-resolved properties of emission enhancement in polar/semi-polar InGaN/GaN by surface plasmon resonance.

作者信息

Ikeda Kento, Kawai Kanata, Kametani Jun, Matsuyama Tetsuya, Wada Kenji, Okada Narihito, Tadatomo Kazuyuki, Okamoto Koichi

机构信息

Department of Physics and Electronics, Osaka Metropolitan University, Gakuen-cho, Naka-ku, Sakai-shi, Osaka 599-8531, Japan.

Department of Electrical and Electronic Engineering, Yamaguchi University, Tokiwadai, Ube-shi, Yamaguchi 755-8611, Japan.

出版信息

Nanophotonics. 2024 Feb 7;13(8):1435-1447. doi: 10.1515/nanoph-2023-0758. eCollection 2024 Apr.

Abstract

Light-emitting diodes (LEDs) are widely used as next-generation light sources because of their various advantages. However, their luminous efficiency is remarkably low at the green-emission wavelength. The luminous efficiencies of InGaN/GaN quantum wells (QWs) significantly decrease with increasing indium content in the green wavelength region, mainly owing to the quantum-confined Stark effect (QCSE). This green gap problem can be solved using QWs grown on semi-polar GaN substrates, such as the {11-22} planes, to reduce the QCSE. We propose that the use of surface plasmons (SPs) is a promising way to improve the light emission efficiency of light-emitting materials such as InGaN/GaN QWs. SP resonance increases the spontaneous emission rates of the excited states, causes a relative reduction in non-radiative relaxation, and ultimately increases the internal quantum efficiencies. In this study, the light emissions of InGaN/GaN QWs grown on polar and semi-polar GaN were investigated using micro-photoluminescence (PL). We successfully enhanced the light emission of semi-polar GaN via SP resonance. The PL peak intensities and wavelengths were mapped and compared to determine the underlying mechanisms. We also measured the emission lifetimes by time-resolved PL and interpreted the detailed mechanism of SP-enhanced emissions. It was found that SP resonances can control not only the emission efficiency but also the exciton dynamics, such as exciton localization effects, QCSE screening, and defect level saturation. We conclude that the green gap problem can be solved by SP-enhanced light emission in semipolar InGaN/GaN.

摘要

发光二极管(LED)因其诸多优点而被广泛用作下一代光源。然而,它们在绿色发射波长处的发光效率极低。在绿色波长区域,InGaN/GaN量子阱(QW)的发光效率随着铟含量的增加而显著降低,这主要归因于量子限制斯塔克效应(QCSE)。使用在半极性GaN衬底(如{11-22}面)上生长的量子阱可以解决这个绿色差距问题,以降低QCSE。我们提出,利用表面等离子体(SP)是提高InGaN/GaN量子阱等发光材料发光效率的一种很有前景的方法。SP共振提高了激发态的自发发射速率,相对减少了非辐射弛豫,并最终提高了内量子效率。在本研究中,使用微光致发光(PL)研究了在极性和半极性GaN上生长的InGaN/GaN量子阱的发光情况。我们通过SP共振成功增强了半极性GaN的发光。绘制并比较了PL峰强度和波长,以确定其潜在机制。我们还通过时间分辨PL测量了发射寿命,并解释了SP增强发射的详细机制。结果发现,SP共振不仅可以控制发射效率还可以控制激子动力学,如激子局域化效应、QCSE屏蔽和缺陷能级饱和。我们得出结论,半极性InGaN/GaN中SP增强的发光可以解决绿色差距问题。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a567/11635936/d155c338f717/j_nanoph-2023-0758_fig_001.jpg

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