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通过脉冲激光照射胶体金纳米颗粒实现纳米气泡成核

Nanobubble nucleation by pulsed laser illumination of colloidal gold nanoparticles.

作者信息

Sharma Yatha, Ohl Claus-Dieter, Rosselló Juan Manuel

机构信息

Institute of Physics, Soft Matter Department, Otto-von-Guericke University, Universitätsplatz 2, 39106, Magdeburg, Germany.

Faculty of Mechanical Engineering, University of Ljubljana, Aškerčeva 6, 1000, Ljubljana, Slovenia.

出版信息

Sci Rep. 2024 Dec 16;14(1):30491. doi: 10.1038/s41598-024-81831-y.

Abstract

This study expands upon a technique our team previously developed for generating nanobubbles on demand with a collimated pulsed laser beam. This work highlights how the controlled addition of gold nanoparticles enhances nanobubble generation efficiency in water, even at laser intensities well below the threshold for multiphoton ionization. Specifically, we investigated the influence of nanoparticles of three distinct sizes on the laser fluence threshold for bubble nucleation and the lifetime of the resultant nanobubbles. Our findings confirm that nanoparticles with a diameter of 60 nm exhibit the greatest nucleation efficiency, achieving nearly 45 % at a fluence threshold of around [Formula: see text]. Interestingly, nanoparticle size did not impact the nanobubble lifetime.

摘要

本研究扩展了我们团队之前开发的一种技术,即利用准直脉冲激光束按需产生纳米气泡。这项工作突出了可控添加金纳米颗粒如何提高水中纳米气泡的产生效率,即使在远低于多光子电离阈值的激光强度下也是如此。具体而言,我们研究了三种不同尺寸的纳米颗粒对气泡成核的激光能量密度阈值以及所得纳米气泡寿命的影响。我们的研究结果证实,直径为60纳米的纳米颗粒表现出最高的成核效率,在约[公式:见正文]的能量密度阈值下达到近45%。有趣的是,纳米颗粒尺寸并未影响纳米气泡的寿命。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/93b1/11649781/af3d68bf7bfc/41598_2024_81831_Fig1_HTML.jpg

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