Zou Chen, Cao Xuhui, Wang Zixiang, Yang Yichen, Lian Yaxiao, Zhao Baodan, Di Dawei
State Key Laboratory of Extreme Photonics and Instrumentation, College of Optical Science and Engineering, International Research Center for Advanced Photonics, Zhejiang University, Hangzhou 310027, China.
Sci Adv. 2025 Jan 10;11(2):eadr8826. doi: 10.1126/sciadv.adr8826.
Solution-processed semiconductor lasers are next-generation light sources for large-scale, bio-compatible and integrated photonics. However, overcoming their performance-cost trade-off to rival III-V laser functionalities is a long-standing challenge. Here, we demonstrate room-temperature continuous-wave perovskite polariton lasers exhibiting remarkably low thresholds of ~0.4 W cm, enabled by a variable single-crystal perovskite microcavity. The threshold outperforms state-of-the-art III-V lasers by ~30 times under optical pumping, and is exceptional among solution-processed lasers. The ultralow-threshold lasing arises from steady-state exciton-polariton condensation, a macroscopic quantum phenomenon akin to Bose-Einstein condensation. The steady-state condensation is attained by fine-tuning the cavity photon-exciton energy separation near the degeneracy point for strong light-matter interactions. These mechanisms enabled the initial demonstration of an indirectly injected perovskite laser chip powered by a gallium nitride light-emitting diode. Our findings create exciting avenues toward on-chip integration of solution-processed lasers, opening opportunities for lasing with ultralow energy consumption and unprecedented performance.
溶液处理的半导体激光器是用于大规模、生物兼容和集成光子学的下一代光源。然而,克服其性能与成本之间的权衡以媲美III-V族激光功能是一个长期存在的挑战。在此,我们展示了室温连续波钙钛矿极化激元激光器,其通过可变单晶钙钛矿微腔实现了约0.4 W/cm的极低阈值。在光泵浦下,该阈值比最先进的III-V族激光器优约30倍,在溶液处理的激光器中表现卓越。超低阈值激光发射源于稳态激子-极化激元凝聚,这是一种类似于玻色-爱因斯坦凝聚的宏观量子现象。通过在简并点附近微调腔光子-激子能量分离以实现强光-物质相互作用,从而实现稳态凝聚。这些机制促成了由氮化镓发光二极管驱动的间接注入钙钛矿激光芯片的首次演示。我们的发现为溶液处理激光器的片上集成开辟了令人兴奋的途径,为超低能耗和前所未有的性能的激光发射创造了机会。