Yang Weimin, Wang Jingyu, He Yonglin, Jiang Shengjie, Hou Liling, Zhuo Liqiang
School of Electronic Information, Zhangzhou Institute of Technology, Zhangzhou 363000, China.
School of Physics and Information Engineering, Shanxi Normal University, Taiyuan 030000, China.
Nanoscale. 2024 Mar 21;16(12):6068-6077. doi: 10.1039/d4nr00042k.
The exciton-polaritons in a lead halide perovskite not only have great significance for macroscopic quantum effects but also possess vital potential for applications in ultralow-threshold polariton lasers, integrated photonics, slow-light devices, and quantum light sources. In this study, we have successfully demonstrated strong coupling with huge Rabi splitting of 553 meV between perovskite excitons and anapole modes in the perovskite metasurface at room temperature. This outcome is achieved by introducing anapole modes to suppress radiative losses, thereby confining light to the perovskite metasurface and subsequently hybridizing it with excitons in the same material. Our results indicate the formation of self-hybridized exciton-polaritons within the perovskite metasurface, which may pave the way towards achieving high coupling strengths that could potentially bring exciting phenomena to fruition, such as Bose-Einstein condensation as well as enabling applications such as efficient light-emitting diodes and lasers.
卤化铅钙钛矿中的激子极化激元不仅对宏观量子效应具有重要意义,而且在超低阈值极化激元激光器、集成光子学、慢光器件和量子光源等应用方面具有至关重要的潜力。在本研究中,我们成功地证明了在室温下,钙钛矿激子与钙钛矿超表面中的暗极子模式之间存在强耦合,拉比分裂高达553毫电子伏特。这一结果是通过引入暗极子模式来抑制辐射损耗实现的,从而将光限制在钙钛矿超表面,并随后使其与同一材料中的激子杂交。我们的结果表明在钙钛矿超表面内形成了自杂交激子极化激元,这可能为实现高耦合强度铺平道路,而高耦合强度可能会使诸如玻色-爱因斯坦凝聚等令人兴奋的现象成为现实,并实现诸如高效发光二极管和激光器等应用。