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5.0° 扭转双层 WSe₂ 中的超导性

Superconductivity in 5.0° twisted bilayer WSe.

作者信息

Guo Yinjie, Pack Jordan, Swann Joshua, Holtzman Luke, Cothrine Matthew, Watanabe Kenji, Taniguchi Takashi, Mandrus David G, Barmak Katayun, Hone James, Millis Andrew J, Pasupathy Abhay, Dean Cory R

机构信息

Department of Physics, Columbia University, New York, NY, USA.

Department of Applied Physics and Applied Mathematics, Columbia University, New York, NY, USA.

出版信息

Nature. 2025 Jan;637(8047):839-845. doi: 10.1038/s41586-024-08381-1. Epub 2025 Jan 22.

Abstract

The discovery of superconductivity in twisted bilayer and trilayer graphene has generated tremendous interest. The key feature of these systems is an interplay between interlayer coupling and a moiré superlattice that gives rise to low-energy flat bands with strong correlations. Flat bands can also be induced by moiré patterns in lattice-mismatched and/or twisted heterostructures of other two-dimensional materials, such as transition metal dichalcogenides (TMDs). Although a wide range of correlated phenomena have indeed been observed in moiré TMDs, robust demonstration of superconductivity has remained absent. Here we report superconductivity in 5.0° twisted bilayer WSe with a maximum critical temperature of 426 mK. The superconducting state appears in a limited region of displacement field and density that is adjacent to a metallic state with a Fermi surface reconstruction believed to arise from AFM order. A sharp boundary is observed between the superconducting and magnetic phases at low temperature, reminiscent of spin fluctuation-mediated superconductivity. Our results establish that moiré flat-band superconductivity extends beyond graphene structures. Material properties that are absent in graphene but intrinsic among TMDs, such as a native band gap, large spin-orbit coupling, spin-valley locking and magnetism, offer the possibility of accessing a broader superconducting parameter space than graphene-only structures.

摘要

扭曲双层和三层石墨烯中超导电性的发现引起了极大的关注。这些体系的关键特征是层间耦合与莫尔超晶格之间的相互作用,这种相互作用产生了具有强关联的低能平带。在其他二维材料(如过渡金属二卤化物(TMDs))的晶格失配和/或扭曲异质结构中的莫尔图案也能诱导出平带。尽管在莫尔TMDs中确实观察到了广泛的关联现象,但超导电性的有力证明仍然缺乏。在此,我们报道了5.0°扭曲双层WSe₂中的超导电性,其最高临界温度为426 mK。超导态出现在位移场和密度的有限区域,该区域与一个金属态相邻,该金属态具有据信由反铁磁序引起的费米面重构。在低温下,超导相和磁相之间观察到一个清晰的边界,这让人联想到自旋涨落介导的超导电性。我们的结果表明,莫尔平带超导电性超出了石墨烯结构。石墨烯中不存在但TMDs中固有的材料特性,如固有带隙、大自旋轨道耦合、自旋谷锁定和磁性,提供了比仅含石墨烯结构更广阔的超导参数空间的可能性。

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