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hBN覆盖和封装的少层石墨烯中纳米级不均匀性的超分辨率成像

Super-Resolution Imaging of Nanoscale Inhomogeneities in hBN-Covered and Encapsulated Few-Layer Graphene.

作者信息

Jäckering Lina, Wirth Konstantin G, Conrads Lukas, Profe Jonas B, Rothstein Alexander, Kyoseva Hristiyana, Watanabe Kenji, Taniguchi Takashi, Kennes Dante M, Stampfer Christoph, Waldecker Lutz, Taubner Thomas

机构信息

1st Institute of Physics (IA), RWTH Aachen University, 52074, Aachen, Germany.

Juelich-Aachen Research Alliance (JARA-FIT), 52425, Juelich, Germany.

出版信息

Adv Sci (Weinh). 2025 Apr;12(14):e2409039. doi: 10.1002/advs.202409039. Epub 2025 Feb 14.

Abstract

Encapsulating few-layer graphene (FLG) in hexagonal boron nitride (hBN) can cause nanoscale inhomogeneities in the FLG, including changes in stacking domains and topographic defects. Due to the diffraction limit, characterizing these inhomogeneities is challenging. Recently, the visualization of stacking domains in encapsulated four-layer graphene (4LG) has been demonstrated with phonon polariton (PhP)-assisted near-field imaging. However, the underlying coupling mechanism and ability to image subdiffractional-sized inhomogeneities remain unknown. Here, direct replicas and magnified images of subdiffractional-sized inhomogeneities in hBN-covered trilayer graphene (TLG) and encapsulated 4LG, enabled by the hyperlensing effect, are retrieved. This hyperlensing effect is mediated by hBN's hyperbolic PhP that couple to the FLG's plasmon polaritons. Using near-field microscopy, the coupling is identified by determining the polariton dispersion in hBN-covered TLG to be stacking-dependent. This work demonstrates super-resolution and magnified imaging of inhomogeneities, paving the way for the realization of homogeneous encapsulated FLG transport samples to study correlated physics.

摘要

将少层石墨烯(FLG)封装在六方氮化硼(hBN)中会导致FLG中出现纳米级不均匀性,包括堆叠域的变化和形貌缺陷。由于衍射极限,表征这些不均匀性具有挑战性。最近,通过声子极化激元(PhP)辅助的近场成像,已证明了对封装的四层石墨烯(4LG)中堆叠域的可视化。然而,潜在的耦合机制以及对亚衍射尺寸不均匀性进行成像的能力仍然未知。在此,通过超透镜效应获取了hBN覆盖的三层石墨烯(TLG)和封装的4LG中亚衍射尺寸不均匀性的直接复制品和放大图像。这种超透镜效应由hBN的双曲线PhP介导,其与FLG的表面等离激元极化激元耦合。使用近场显微镜,通过确定hBN覆盖的TLG中的极化激元色散与堆叠相关来识别这种耦合。这项工作展示了不均匀性的超分辨率和放大成像,为实现用于研究相关物理的均匀封装FLG传输样品铺平了道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f6ae/11984919/24fa5eb00658/ADVS-12-2409039-g005.jpg

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