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提高接触电催化效率的策略:综述

Strategies for Improving Contact-Electro-Catalytic Efficiency: A Review.

作者信息

Liu Meng-Nan, Liu Jin-Hua, Wang Lu-Yao, Yin Fang, Zheng Gang, Li Ru, Zhang Jun, Long Yun-Ze

机构信息

Collaborative Innovation Center for Nanomaterials & Devices, Innovation Institute for Advanced Nanofibers, College of Physics, Qingdao University, Qingdao 266071, China.

Instrumental Analysis Center of Qingdao University, Qingdao 266071, China.

出版信息

Nanomaterials (Basel). 2025 Mar 2;15(5):386. doi: 10.3390/nano15050386.

DOI:10.3390/nano15050386
PMID:40072189
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11901548/
Abstract

Contact-electro-catalysis (CEC) has emerged as a promising catalytic methodology, integrating principles from solid-liquid triboelectric nanogenerators (SL-TENGs) into catalysis. Unlike conventional approaches, CEC harnesses various forms of mechanical energy, including wind and water, along with other renewable sources, enabling reactions under natural conditions without reliance on specific energy inputs like light or electricity. This review presents the basic principles of CEC and discusses its applications, including the degradation of organic molecules, synthesis of chemical substances, and reduction of metals. Furthermore, it explores methods to improve the catalytic efficiency of CEC by optimizing catalytic conditions, the structure of catalyst materials, and the start-up mode. The concluding section offers insights into future prospects and potential applications of CEC, highlighting its role in advancing sustainable catalytic technologies.

摘要

接触电催化(CEC)已成为一种很有前景的催化方法,它将固液摩擦纳米发电机(SL-TENGs)的原理融入催化过程。与传统方法不同,CEC利用包括风能和水能在内的各种形式的机械能以及其他可再生能源,使反应能够在自然条件下进行,而无需依赖光或电等特定能量输入。本文综述了CEC的基本原理,并讨论了其应用,包括有机分子的降解、化学物质的合成以及金属的还原。此外,还探讨了通过优化催化条件、催化剂材料结构和启动模式来提高CEC催化效率的方法。结论部分对CEC的未来前景和潜在应用进行了展望,突出了其在推动可持续催化技术发展中的作用。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/9214d9da03c3/nanomaterials-15-00386-g012.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/8e572f2a814b/nanomaterials-15-00386-g011.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/83c19fa7c07a/nanomaterials-15-00386-g003.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/fc1601ab3c74/nanomaterials-15-00386-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/d148c27b5883/nanomaterials-15-00386-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/832ae88dc10b/nanomaterials-15-00386-g008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/a70f8ab127bd/nanomaterials-15-00386-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/08073e292c0f/nanomaterials-15-00386-g010.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/8e572f2a814b/nanomaterials-15-00386-g011.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf46/11901548/9214d9da03c3/nanomaterials-15-00386-g012.jpg

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本文引用的文献

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A wearable triboelectric impedance tomography system for noninvasive and dynamic imaging of biological tissues.一种用于生物组织无创动态成像的可穿戴摩擦电阻抗断层扫描系统。
Sci Adv. 2024 Dec 20;10(51):eadr9139. doi: 10.1126/sciadv.adr9139.
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Triboelectric sensor with ultra-wide linear range based on water-containing elastomer and ion-rich interface.基于含水弹性体和富离子界面的超宽线性范围摩擦电传感器。
Nat Commun. 2024 Dec 6;15(1):10640. doi: 10.1038/s41467-024-54980-x.
3
Regulating Contact-Electro-Catalysis Using Polymer/Metal Janus Composite Catalysts.
使用聚合物/金属双面复合催化剂调控接触电催化
J Am Chem Soc. 2024 Oct 1. doi: 10.1021/jacs.4c07446.
4
Boosting Reactive Oxygen Species Generation via Contact-Electro-Catalysis with Fe-Initiated Self-cycled Fenton System.通过与铁引发的自循环芬顿体系进行接触电催化增强活性氧生成
Angew Chem Int Ed Engl. 2025 Jan 2;64(1):e202413246. doi: 10.1002/anie.202413246. Epub 2024 Oct 18.
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Contact-Electro-Catalysis Through Electret Behavior to Facilitate Electron Transfer.通过驻极体行为实现接触电催化以促进电子转移。
ACS Appl Mater Interfaces. 2024 Aug 14;16(32):42293-42304. doi: 10.1021/acsami.4c09206. Epub 2024 Aug 5.
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Contact-electro-catalytic CO reduction from ambient air.从环境空气中进行接触电催化CO还原。
Nat Commun. 2024 Jul 13;15(1):5913. doi: 10.1038/s41467-024-50118-1.
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Reduction of precious metal ions in aqueous solutions by contact-electro-catalysis.通过接触电催化还原水溶液中的贵金属离子。
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Simultaneous Cu(II)-EDTA decomplexation and Cu(II) recovery using integrated contact-electro-catalysis and capacitive deionization from electroplating wastewater.利用集成接触电催化和电容去离子技术从电镀废水中同步进行Cu(II)-EDTA解络和Cu(II)回收
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Contact-electro-catalysis (CEC).接触电催化(CEC)。
Chem Soc Rev. 2024 May 7;53(9):4349-4373. doi: 10.1039/d3cs00736g.
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Contact-Electro-Catalysis for Direct Oxidation of Methane under Ambient Conditions.环境条件下甲烷直接氧化的接触电催化
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