Li Yue, Nabi Md Rafique Un, Park Hyowon, Liu Yuzi, Rosenkranz Stephan, Petford-Long Amanda K, Hu Jin, Velthuis Suzanne G E Te, Phatak Charudatta
Materials Science Division, Argonne National Laboratory, Lemont, IL, 60439, USA.
Department of Physics, University of Arkansas, Fayetteville, AR, 72701, USA.
Small. 2025 Apr;21(17):e2406299. doi: 10.1002/smll.202406299. Epub 2025 Mar 20.
Ferrimagnets, which have both ferromagnetic and antiferromagnetic coupling, are attracting increased attention in the realm of spintronic devices due to advantages such as ultrafast dynamics and a suppressed skyrmion Hall effect. Thus, understanding the behavior of nontrivial spin textures in ferrimagnets is crucial; however, comprehensive reports on this topic remain limited. Here, the magnetic spin textures of ferrimagnetic MnZnSb (x = 0.85) is explored as a function of temperature and applied magnetic field. The spin textures can be tuned to a variety of states, including stripes, skyrmion bags, and a skyrmion lattice. Chiral Néel-type magnetic structures are visualized using Lorentz transmission electron microscopy. Mn(I) ions are slightly shifted toward the Sb sites, which may be due to a strong electrostatic interaction between Mn and Sb ions. This local structural distortion breaks the inversion symmetry and introduces an effective Dzyaloshinkii-Moriya interaction. This work thus provides a pathway to use doping and heterogeneity in a ferrimagnet to control and generate chiral nontrivial spin textures.
具有铁磁和反铁磁耦合的亚铁磁体,由于具有超快动力学和抑制的斯格明子霍尔效应等优点,在自旋电子器件领域正受到越来越多的关注。因此,了解亚铁磁体中非平凡自旋纹理的行为至关重要;然而,关于这一主题的全面报道仍然有限。在此,研究了亚铁磁体MnZnSb(x = 0.85)的磁自旋纹理随温度和外加磁场的变化。自旋纹理可以被调节到各种状态,包括条纹、斯格明子袋和斯格明子晶格。使用洛伦兹透射电子显微镜观察到手性奈尔型磁结构。Mn(I)离子向Sb位点略有偏移,这可能是由于Mn和Sb离子之间强烈的静电相互作用。这种局部结构畸变打破了反演对称性,并引入了有效的Dzyaloshinkii-Moriya相互作用。因此,这项工作提供了一条利用亚铁磁体中的掺杂和不均匀性来控制和产生手性非平凡自旋纹理的途径。