Sharma Priyanka, Yuan Hao, Verma Ruchi, Mehla Nisha, Hemant Hemant, Sagar Poonam, Comby-Zerbino Clothilde, Russier-Antoine Isabelle, Moulin Christophe, Brevet Pierre-François, Singhal Nitin, Neelakandan Prakash P, Vaidya Sonalika, Fu Changkui, Ali Md Ehesan, Srivastava Rohit, Whittaker Andrew, Antoine Rodolphe, Shanavas Asifkhan
Inorganic & Organic Nanomedicine (ION) Lab, Institute of Nano Science and Technology (INST), Sector 81, Knowledge City, Mohali, Punjab, 140306, India.
Institut Lumière Matière (ILM) UMR 5306, Université Claude Bernard Lyon 1, CNRS, Univ Lyon, Villeurbanne, F-69100, France.
Adv Healthc Mater. 2025 Jun;14(15):e2405005. doi: 10.1002/adhm.202405005. Epub 2025 Mar 20.
Intrinsically theranostic metal nanoclusters are rare unless the stabilizing ligands exhibit therapeutic properties. A promising class of quasi-molecular, near-infrared (NIR) emitting, cytotoxic gold nanoclusters, coined as AXE (Au eXcitable and Eliminable) stabilized through terminal thioester groups on fluorinated, and crosslinked polymers, is presented for simultaneous bioimaging & therapy. Nano Variable Temperature-Electrospray ionization mass spectrometry analysis of these aqueous stable nanoclusters revealed 5 to 7 core gold atoms, with SAXS measurement confirming average size to be under 1 nm, consistent with the theoretical maximum for few atom planar gold clusters. Despite its small size, AXE exhibits a remarkable Stoke shift of ≈470 nm and emission range spanning 700 to 1100 nm. Fluorination notably enhanced the quantum yield by up to twofold, attributed to charge transfer from the fluorinated monomer to the gold core, as indicated by Löwdin charge distribution analysis. The AXE nanocluster demonstrated dose-dependent pro-apoptotic effects on cancer cells while sparing normal cells at lower concentrations. Preclinical evaluation in a breast tumor model confirmed its anticancer efficacy, with intravenous and intraperitoneal administrations significantly inhibiting tumor growth and controlling lung metastasis, surpassing the clinical standard, doxorubicin.
除非稳定配体具有治疗特性,否则具有内在诊疗功能的金属纳米团簇很少见。本文介绍了一类有前景的准分子、近红外(NIR)发射、具有细胞毒性的金纳米团簇,称为AXE(可激发和可消除的金),它通过氟化交联聚合物上的末端硫酯基团稳定,可用于同时进行生物成像和治疗。对这些水相稳定纳米团簇的纳米可变温度-电喷雾电离质谱分析显示有5至7个核心金原子,小角X射线散射测量证实平均尺寸小于1纳米,这与少数原子平面金团簇的理论最大值一致。尽管AXE尺寸小,但它具有约470纳米的显著斯托克斯位移,发射范围为700至1100纳米。氟化显著提高了量子产率,最高可达两倍,如洛丁电荷分布分析所示,这归因于从氟化单体到金核的电荷转移。AXE纳米团簇对癌细胞表现出剂量依赖性促凋亡作用,而在较低浓度下对正常细胞无影响。在乳腺肿瘤模型中的临床前评估证实了其抗癌功效,静脉内和腹腔内给药均能显著抑制肿瘤生长并控制肺转移,超过临床标准药物阿霉素。