Aslam Junaid, Waseem Muhammad Ahsan, Wu Yibo, Sun Weiwei, Wang Yong
Department of Chemical Engineering, School of Environmental and Chemical Engineering, Shanghai University, 99 Shangda Road, Shanghai 200444, PR China.
Department of Chemical Engineering, School of Environmental and Chemical Engineering, Shanghai University, 99 Shangda Road, Shanghai 200444, PR China; Key Laboratory of Organic Compound Pollution Control Engineering (MOE), Shanghai University, 99 Shangda Road, Shanghai 200444, PR China.
Adv Colloid Interface Sci. 2025 Jul;341:103479. doi: 10.1016/j.cis.2025.103479. Epub 2025 Mar 19.
The escalating demand for sustainable energy storage solutions has spurred significant research into materials that can efficiently store and convert energy. Among these, Covalent Triazine Frameworks (CTFs) have emerged as a promising class of two-dimensional nanomaterials due to their unique properties which includes permanent porosity, abundant active sites, exceptional stability and structural diversity. This review examines the role of CTFs in enhancing the performance of electrochemical energy storage devices, particularly in LIBs and LSBs as electrode materials. Despite the advantages of CTFs based electrode materials, such as their lightweight nature, design flexibility, and sustainability, they often suffer from low ionic conductivity and durability issues. This review examines recent advancements and design approaches focused on enhancing the electrochemical performance of CTF-based electrodes for lithium-ion (LIBs) and lithium‑sulfur (LSBs) batteries. It also addresses the major challenges that limit the effectiveness of CTFs in energy storage applications and suggests potential strategies for overcoming these obstacles. The primary aim of this review is to offer a thorough and detailed overview of the current state of research on CTFs. By critically analyzing existing work and highlighting future research directions, this review intends to support the advancement of CTF-based technologies in pursuit of more efficient and sustainable energy storage solutions.
对可持续储能解决方案不断增长的需求推动了对能够高效存储和转换能量的材料的大量研究。其中，共价三嗪框架（CTF）因其独特的性质，包括永久孔隙率、丰富的活性位点、出色的稳定性和结构多样性，已成为一类有前途的二维纳米材料。本文综述了CTF在提高电化学储能装置性能方面的作用，特别是在作为锂离子电池（LIB）和锂硫电池（LSB）电极材料方面。尽管基于CTF的电极材料具有诸如轻质、设计灵活性和可持续性等优点，但它们常常存在离子电导率低和耐久性问题。本文综述了近期专注于提高基于CTF的锂离子电池（LIB）和锂硫电池（LSB）电极电化学性能的进展和设计方法。它还讨论了限制CTF在储能应用中有效性的主要挑战，并提出了克服这些障碍的潜在策略。本文综述的主要目的是全面、详细地概述CTF的当前研究现状。通过批判性地分析现有工作并突出未来研究方向，本文综述旨在支持基于CTF的技术发展，以寻求更高效、可持续的储能解决方案。
