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俄勒冈州农村非催化薪柴炉排放和燃料装载量的现场测量。

In-situ measurements of emissions and fuel loading of non-catalytic cordwood stoves in rural Oregon.

作者信息

Bentson Samuel, Thompson Ryan, Berger Jaden, Wald Jonah, MacCarty Nordica

机构信息

Aprovecho Research Center, Cottage Grove, Oregon, USA.

Mountain Air Engineering, Cottage Grove, Oregon, USA.

出版信息

J Air Waste Manag Assoc. 2025 Jul;75(7):503-521. doi: 10.1080/10962247.2025.2483217. Epub 2025 May 14.

DOI:10.1080/10962247.2025.2483217
PMID:40146210
Abstract

Residential wood combustion is an important source of heat for millions of households, yet it represents the third largest source of PM pollution in the United States. Development of cleaner-burning cordwood heating stove designs is necessary to reduce health and climate impacts from this important renewable energy source. Effective design requires an understanding of operation and performance of existing stoves in real-world settings. In this study, one uncertified stove, three EPA Phase I or II stoves, and three New Source Performance Standards (NSPS) stoves were sampled for 48 consecutive hours each in households in rural Oregon. The methodology included stack sampling of undiluted CO and CO with a diluted sample train for cooling and condensation of PM and an optical sensor to apportion integrated gravimetric measurements of particle mass over time. A data-logging scale directly measured fuel loading mass and timing, enabling emissions mass calculations via both stack flow and carbon balance methods. Results across all stoves showed that together cold starts and reloads contribute 70% of total PM emissions. The measured period emission rate of PM over all stoves was 5.6 ± 2.2 g/hr, while the average emission factor of PM was 8.5 ± 3.0 g/kg. There was a statistically significant reduction of between 29.6-48.5% in the PM emission rate during all periods except burnout and a 40.6 increase in thermal efficiency of the NSPS stoves relative to the single uncertified stove during the fire period. Implications of this study include both a database of in-field emissions and efficiency performance measures and comparison of stove certification levels that are useful to wood stove designers and policymakers for optimizing air quality impacts of stove-user systems. In addition, the methods demonstrated here can be used by researchers to promote needed field monitoring capabilities at a lower cost and complexity.: Detailed time-apportioned PM emissions data identified conditions leading to high emission rates including startup, large loads, and operation of an uncertified stove. Provides wood stove designers insights toward optimizing performance of future stove designs, and policy makers information about the impact of user and technology on air quality objectives. Demonstrated new equipment for real-time emissions and fuel consumption monitoring that enables time-resolved PM and direct fuel mass measurements to yield better design insights for heating stoves. This method can be used by other researchers to gather much needed field measurements at a lower cost and complexity than existing methods.

摘要

住宅用木柴燃烧是数百万家庭重要的取暖热源,但它却是美国第三大细颗粒物污染来源。开发更清洁燃烧的薪柴取暖炉设计对于减少这一重要可再生能源对健康和气候的影响很有必要。有效的设计需要了解现有炉灶在实际环境中的运行和性能。在本研究中,在俄勒冈州农村的家庭中,对一台未经认证的炉灶、三台美国环境保护局(EPA)第一阶段或第二阶段炉灶以及三台新源性能标准(NSPS)炉灶分别进行了连续48小时的采样。该方法包括用未稀释的一氧化碳(CO)和经稀释的采样系统采集的CO进行烟囱采样,以冷却和冷凝细颗粒物,并使用光学传感器按时间分配颗粒物质量的综合重量测量值。一个数据记录秤直接测量燃料装载量和时间,从而能够通过烟囱流量和碳平衡方法计算排放质量。所有炉灶的结果表明,冷启动和重新装填共同造成了70%的细颗粒物总排放。所有炉灶的细颗粒物测量期间排放率为5.6±2.2克/小时,而细颗粒物的平均排放因子为8.5±3.0克/千克。除了燃尽阶段外,所有阶段的细颗粒物排放率在统计上显著降低了29.6 - 48.5%,并且在燃烧期间,NSPS炉灶的热效率相对于单一未经认证的炉灶提高了40.6%。本研究的意义包括一个现场排放和效率性能测量的数据库,以及炉灶认证水平的比较,这对木柴炉灶设计师和政策制定者优化炉灶 - 用户系统对空气质量的影响很有用。此外,这里展示的方法可供研究人员以更低的成本和复杂度用于提升所需的现场监测能力。详细的按时间分配的细颗粒物排放数据确定了导致高排放率的条件,包括启动、大负荷以及未经认证炉灶的运行。为木柴炉灶设计师提供了优化未来炉灶设计性能的见解,并为政策制定者提供了有关用户和技术对空气质量目标影响的信息。展示了用于实时排放和燃料消耗监测的新设备,该设备能够进行时间分辨的细颗粒物和直接燃料质量测量,从而为取暖炉提供更好的设计见解。这种方法可供其他研究人员以比现有方法更低的成本和复杂度收集急需的现场测量数据。

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